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处于与其子体平衡状态的锕衰变过程中绝对γ射线发射概率的测量。

Measurement of absolute γ-ray emission probabilities in the decay of Ac in equilibrium with its progeny.

作者信息

Marouli M, Lutter G, Pommé S, Van Ammel R, Hult M, Pierre S, Dryák P, Carconi P, Fazio A, Bruchertseifer F, Morgenstern A

机构信息

European Commission, Joint Research Centre, Directorate for Nuclear Safety and Security, Retieseweg 111, B-2440 Geel, Belgium.

CEA, LIST, Laboratoire National Henri Becquerel (LNE-LNHB), Bât. 602 PC111 CEA Saclay, F-91191 Gif-sur-Yvette, France.

出版信息

Appl Radiat Isot. 2019 Feb;144:34-46. doi: 10.1016/j.apradiso.2018.08.023. Epub 2018 Aug 30.

DOI:10.1016/j.apradiso.2018.08.023
PMID:30522082
Abstract

The emission probabilities of γ rays produced in the Ac decay series were determined by high-resolution γ-ray spectrometry of sources with standardised activity. The sources were prepared quantitatively on glass discs by drop deposition of a solution with Ac in radioactive equilibrium with its daughter nuclides. Their activity was measured by a primary standardisation technique based on alpha-particle counting at a defined low solid angle. Four laboratories performed γ-ray spectrometry and derived absolute γ-ray intensities. Mean values were calculated and compared with literature data and the currently recommended evaluated data. New values on certain γ-ray emission probabilities are proposed.

摘要

通过对具有标准化活度的源进行高分辨率γ射线能谱分析,确定了锕衰变系列中产生的γ射线的发射概率。通过滴加含有与其子核素处于放射性平衡的锕的溶液,在玻璃盘上定量制备源。通过基于在定义的低立体角下进行α粒子计数的初级标准化技术测量它们的活度。四个实验室进行了γ射线能谱分析并得出了绝对γ射线强度。计算了平均值,并与文献数据和当前推荐的评估数据进行了比较。提出了某些γ射线发射概率的新值。

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