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热传导中的声子局域化。

Phonon localization in heat conduction.

作者信息

Luckyanova M N, Mendoza J, Lu H, Song B, Huang S, Zhou J, Li M, Dong Y, Zhou H, Garlow J, Wu L, Kirby B J, Grutter A J, Puretzky A A, Zhu Y, Dresselhaus M S, Gossard A, Chen G

机构信息

Department of Mechanical Engineering, Massachusetts Institute of Technology, Cambridge, MA 02139, USA.

Materials Department, University of California, Santa Barbara, Santa Barbara, CA 93106, USA.

出版信息

Sci Adv. 2018 Dec 21;4(12):eaat9460. doi: 10.1126/sciadv.aat9460. eCollection 2018 Dec.

Abstract

Nondiffusive phonon thermal transport, extensively observed in nanostructures, has largely been attributed to classical size effects, ignoring the wave nature of phonons. We report localization behavior in phonon heat conduction due to multiple scattering and interference events of broadband phonons, by measuring the thermal conductivities of GaAs/AlAs superlattices with ErAs nanodots randomly distributed at the interfaces. With an increasing number of superlattice periods, the measured thermal conductivities near room temperature increased and eventually saturated, indicating a transition from ballistic to diffusive transport. In contrast, at cryogenic temperatures the thermal conductivities first increased but then decreased, signaling phonon wave localization, as supported by atomistic Greenșs function simulations. The discovery of phonon localization suggests a new path forward for engineering phonon thermal transport.

摘要

在纳米结构中广泛观察到的非扩散声子热输运,很大程度上归因于经典尺寸效应,而忽略了声子的波动性质。我们通过测量在界面处随机分布有ErAs纳米点的GaAs/AlAs超晶格的热导率,报道了由于宽带声子的多次散射和干涉事件导致的声子热传导中的局域化行为。随着超晶格周期数的增加,在室温附近测得的热导率增加并最终饱和,表明从弹道输运向扩散输运的转变。相比之下,在低温下,热导率首先增加但随后降低,这表明声子波局域化,原子格林函数模拟也证实了这一点。声子局域化的发现为工程化声子热输运指明了一条新的道路。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/c760/6303120/c0f8d9aa6b6c/aat9460-F1.jpg

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