Duan Shi-Guang, Jiang Nan, Yang Liu-Ming, Zhang Rui-Qin
College of Chemistry and Molecular Engineering, Zhengzhou University, Zhengzhou 450001, China.
Research Institute of Environmental Science, Zhengzhou University, Zhengzhou 450001, China.
Huan Jing Ke Xue. 2019 Jan 8;40(1):86-93. doi: 10.13227/j.hjkx.201805187.
In this study, meteorological and air mass concentration data of Zhengzhou from December 2017 to February 2018 (winter) were used to quantify the influence of meteorological factors on the PM. The Hybrid Single-Particle Lagrangian Integrated Trajectory model was used to analyze the 48-hour backward trajectories and the cluster method was applied to classify the airflow backward trajectory. Moreover, the potential source contribution function and concentration-weighted trajectory analysis were applied to evaluate the transport pathways and sources of PM in Zhengzhou. The results show that the heavy pollution in Zhengzhou during winter is mainly due to the low wind speed, high relative humidity, and low precipitation. The cluster analysis revealed that up to 60% of the back trajectories came from the northwest and 25.56% of the back trajectories came from the Beijing-Tianjin area. The airflow trajectories from the south and east account for 7.5% and 6.1% with higher PM concentrations. The main potential sources of PM in Zhengzhou during winter are located in Beijing-Tianjin-Hebei air pollution transmission channel cities including Jiaozuo, Kaifeng, Xinxiang, Hebi, Puyang, Anyang, Handan, and Xingtai. The adjacent provinces, including Shanxi, Hubei, and Anhui, also have great influence on the PM in Zhengzhou.
本研究利用2017年12月至2018年2月(冬季)郑州的气象和空气质量浓度数据,量化气象因素对颗粒物(PM)的影响。采用混合单粒子拉格朗日积分轨迹模型分析48小时后向轨迹,并运用聚类方法对气流后向轨迹进行分类。此外,应用潜在源贡献函数和浓度加权轨迹分析来评估郑州PM的传输路径和来源。结果表明,郑州冬季的重污染主要归因于低风速、高相对湿度和低降水量。聚类分析显示,高达60%的后向轨迹来自西北方向,25.56%的后向轨迹来自京津地区。来自南方和东方的气流轨迹分别占7.5%和6.1%,其PM浓度较高。郑州冬季PM的主要潜在来源位于京津冀大气污染传输通道城市,包括焦作、开封、新乡、鹤壁、濮阳、安阳、邯郸和邢台。相邻省份,包括山西、湖北和安徽,对郑州的PM也有很大影响。