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[水汽源和局地蒸发对降水稳定氢氧同位素组成的影响]

[Effects of Water Vapor Source and Local Evaporation on the Stable Hydrogen and Oxygen Isotopic Compositions of Precipitation].

作者信息

Hu Yong-Bo, Xiao Wei, Qian Yu-Fei, Liu Qiang, Xie Cheng-Yu, Zhang Xiu-Fang, Zhang Wen-Qing, Wen Xue-Fa, Liu Shou-Dong, Lee Xu-Hui

机构信息

Yale-NUIST Center on Atmospheric Environment, Nanjing University of Information Science and Technology, Nanjing 210044, China.

Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology(CICAEET), Nanjing University of Information Science and Technology, Nanjing 210044, China.

出版信息

Huan Jing Ke Xue. 2019 Feb 8;40(2):573-581. doi: 10.13227/j.hjkx.201805227.

Abstract

Stable hydrogen and oxygen isotopic compositions in precipitation are good tracers and can provide unique information about the water cycle. Precipitation samples were collected at the Nanjing, Liyang, Yixing, and Dongshan sites in 2016, and the HDO and HO compositions of precipitation were measured. The temporal variability of HDO and HO compositions and deuterium-excess of precipitation were analyzed, and the influence of the water vapor source and local evaporation on stable isotopic composition of precipitation were discussed. The results indicated that:① Seasonal variations in the HDO composition, HO composition, and deuterium-excess of precipitation occurred due to different water vapor sources during the summer and winter monsoon seasons. The HDO and HO compositions were depleted during the summer monsoon season and enriched during the winter monsoon season. The deuterium-excess during the summer monsoon season was lower compared to the winter monsoon season. ② During the summer monsoon, the evaporation of Lake Taihu made the deuterium-excess of downwind precipitation and the downwind intercept of the local meteoric water line higher. During the winter monsoon season, local evaporation had little influence on HDO and HO components in precipitation. ③ Both of the intercepts and slopes of the local meteoric water line were higher than those of the global meteoric water line, due to moisture recycling during the winter monsoon season and different water vapor sources between the summer and winter monsoon seasons.

摘要

降水中稳定的氢和氧同位素组成是很好的示踪剂,能够提供有关水循环的独特信息。2016年在南京、溧阳、宜兴和东山站点采集了降水样本,并测定了降水中HDO和H₂O的组成。分析了降水中HDO和H₂O组成以及氘过量的时间变化,并讨论了水汽源和局地蒸发对降水稳定同位素组成的影响。结果表明:①由于夏季风和冬季风季节水汽源不同,降水中HDO组成、H₂O组成和氘过量存在季节变化。夏季风季节HDO和H₂O组成贫化,冬季风季节富集。夏季风季节的氘过量低于冬季风季节。②夏季风期间,太湖蒸发使得下风方向降水的氘过量和局部雨水线的下风截距更高。冬季风季节,局地蒸发对降水中HDO和H₂O组分影响较小。③由于冬季风季节的水汽再循环以及夏季风和冬季风季节不同的水汽源,局部雨水线的截距和斜率均高于全球雨水线。

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