Theoretical Division and Center for Integrated Nanotechnologies, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA.
Nanoscale. 2019 Jan 23;11(4):2037-2047. doi: 10.1039/c8nr02310g.
Understanding the physics of light emitters in quantum nanostructures regarding scalability, geometry, structure of the system and coupling between different degrees of freedom is important as one can improve the design and further provide rigorous controls of quantum devices. The coupling between these degrees of freedom, in general, depends on the external field, the geometry of nano particles, and the experimental design. An effective model is proposed to describe the plasmon-exciton hybrid systems and its optical absorption spectra, which is studied in detail by exact diagonalization. Two different designs are discussed: a nano particle planet surrounded by quantum dot satellites and a quantum dot planet surrounded by nano particle satellites. In both setups, details of many quantum dots and nano particles are studied, and the spectra are discussed in detail regarding the energy of transition peaks and the weight distribution of allowed transition peaks. Also, different polarization of external fields is considered, which results in anisotropic couplings, and the absorption spectra clearly reveal the difference qualitatively. Finally, the system will undergo a phase transition in the presence of attractive interactions between excitons. Our work sheds light on the design of nano scale quantum systems to achieve photon emitter/resonator theory in plasmon-exciton hybrid systems.
理解量子纳米结构中光发射器的物理性质,包括可扩展性、几何形状、系统结构和不同自由度之间的耦合,对于改进设计和进一步提供量子器件的严格控制非常重要。这些自由度之间的耦合通常取决于外部场、纳米粒子的几何形状和实验设计。本文提出了一个有效的模型来描述等离激元-激子混合系统及其光吸收谱,并通过精确对角化对其进行了详细研究。讨论了两种不同的设计:被量子点卫星包围的纳米粒子行星和被纳米粒子卫星包围的量子点行星。在这两种设置中,详细研究了许多量子点和纳米粒子的细节,并详细讨论了跃迁峰的能量和允许跃迁峰的权重分布。此外,还考虑了外部场的不同偏振,这导致各向异性耦合,吸收谱定性地清楚地揭示了这种差异。最后,在激子之间存在吸引力相互作用的情况下,系统将经历相变。我们的工作为设计纳米尺度量子系统提供了启示,以实现等离激元-激子混合系统中的光子发射器/共振器理论。