Centi Gabriele, Čejka Jiří
University of Messina, ERIC aisbl and CASPE/INSTM, Dept.s MIFT-Industrial Chemistry, V.le F. Stagno D'Alcontres 31, 98166, Messina, Italy.
J. Heyrovský Institute of Physical Chemistry, Czech Academy of Science, Dolejškova 3, 182 23, Prague 8, Czech Republic.
ChemSusChem. 2019 Feb 7;12(3):621-632. doi: 10.1002/cssc.201802637. Epub 2019 Jan 16.
Catalysis is undergoing a major transition resulting from significant changes in chemical and energy production. To honor the 50th anniversary of establishing the Jerzy Haber Institute of Catalysis and Surface Chemistry, this Essay discusses, from a forward-looking, personal and somewhat provocative perspective, the needs and gaps of catalysis to address the ongoing transition in chemistry and energy from a sustainability perspective. The focus is on a few selected aspects identified as crucial: i) The precise synthesis of catalytic materials, particularly focusing on mesoporous molecular sieves, metal-organic frameworks, and zeolites (particularly two-dimensional type); ii) advanced catalyst characterization methods; iii) new concepts and approaches needed in catalysis to meet the demands of a field of energy and chemistry in transition.
催化领域正经历着一场重大变革,这源于化学和能源生产方面的显著变化。为纪念耶日·哈伯催化与表面化学研究所成立50周年,本文从前瞻性、个人化且略带挑衅性的视角,探讨了从可持续发展角度看,催化领域应对化学和能源领域当前转型所存在的需求与差距。重点关注几个被视为关键的选定方面:i)催化材料的精确合成,尤其侧重于介孔分子筛、金属有机框架材料和沸石(特别是二维类型);ii)先进的催化剂表征方法;iii)催化领域为满足转型中的能源和化学领域需求所需的新概念和新方法。