Ajoy A, Lv X, Druga E, Liu K, Safvati B, Morabe A, Fenton M, Nazaryan R, Patel S, Sjolander T F, Reimer J A, Sakellariou D, Meriles C A, Pines A
Department of Chemistry, University of California, Berkeley, California 94720, USA.
Materials Science Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA.
Rev Sci Instrum. 2019 Jan;90(1):013112. doi: 10.1063/1.5064685.
We describe the construction of a fast field cycling device capable of sweeping a 4-order-of-magnitude range of magnetic fields, from ∼1 mT to 7 T, in under 700 ms, and which is further extendable to a 1 nT-7 T range. Central to this system is a high-speed sample shuttling mechanism between a superconducting magnet and a magnetic shield, with the capability to access arbitrary fields in between with high resolution. Our instrument serves as a versatile platform to harness the inherent dichotomy of spin dynamics on offer at low and high fields-in particular, the low anisotropy, fast spin manipulation, and rapid entanglement growth at low field as well as the long spin lifetimes, spin specific control, and efficient inductive measurement possible at high fields. Exploiting these complementary capabilities in a single device opens up applications in a host of problems in quantum control, sensing, and information storage, besides in nuclear hyperpolarization, relaxometry, and imaging. In particular, in this paper, we focus on the ability of the device to enable low-field hyperpolarization of C nuclei in diamond via optically pumped electronic spins associated with nitrogen vacancy defect centers.
我们描述了一种快速场循环装置的构建,该装置能够在不到700毫秒的时间内扫描4个数量级范围的磁场,从约1毫特斯拉到7特斯拉,并且还可进一步扩展到1纳特斯拉 - 7特斯拉范围。该系统的核心是一个位于超导磁体和磁屏蔽之间的高速样品穿梭机制,能够以高分辨率访问其间的任意磁场。我们的仪器是一个多功能平台,可利用低场和高场中自旋动力学固有的二分性——特别是低各向异性、快速自旋操纵以及低场下快速的纠缠增长,以及高场下长自旋寿命、自旋特定控制和高效感应测量。在单个设备中利用这些互补能力,除了在核超极化、弛豫测量和成像方面外,还为量子控制、传感和信息存储等一系列问题开辟了应用前景。特别是在本文中,我们重点关注该装置通过与氮空位缺陷中心相关的光泵浦电子自旋实现金刚石中碳核低场超极化的能力。