Max Planck Institute for Solid State Research, Heisenbergstrasse 1, D-70569 Stuttgart, Germany.
Phys Rev Lett. 2019 Feb 8;122(5):057203. doi: 10.1103/PhysRevLett.122.057203.
The consequences of the Jahn-Teller (JT) orbital-lattice coupling for magnetism of pseudospin J_{eff}=1/2 and J_{eff}=0 compounds are addressed. In the former case, represented by Sr_{2}IrO_{4}, this coupling generates, through the so-called pseudo-JT effect, orthorhombic deformations of a crystal concomitant with magnetic ordering. The orthorhombicity axis is tied to the magnetization and rotates with it under magnetic field. The theory resolves a number of puzzles in Sr_{2}IrO_{4} such as the origin of in-plane magnetic anisotropy and magnon gaps, metamagnetic transition, etc. In J_{eff}=0 systems, the pseudo-JT effect leads to spin-nematic transition well above magnetic ordering, which may explain the origin of "orbital order" in Ca_{2}RuO_{4}.
针对赝自旋 J_{eff}=1/2 和 J_{eff}=0 化合物的 Jahn-Teller(JT)轨道-晶格耦合对磁性的影响进行了研究。在以 Sr_{2}IrO_{4} 为代表的前一种情况下,这种耦合通过所谓的赝 JT 效应,在磁有序的同时产生晶体的正交畸变。正交轴与磁化强度相关联,并在磁场下随其旋转。该理论解决了 Sr_{2}IrO_{4} 中的许多难题,例如面内各向异性和磁子能隙、变磁性转变等的起源。在 J_{eff}=0 体系中,赝 JT 效应导致自旋向列相变发生在磁有序之上,这可能解释了 Ca_{2}RuO_{4}中“轨道有序”的起源。