Sølling Theis I, Møller Klaus B
Center for Integrative Petroleum Research, College of Petroleum and Geosciences, King Fahad University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia.
Department of Chemistry, Technical University of Denmark, Kemitorvet 207, 2800 Kgs. Lyngby, Denmark.
Struct Dyn. 2018 Dec 26;5(6):060901. doi: 10.1063/1.5079265. eCollection 2018 Nov.
Coherence is one of the most important phenomena in ultrafast sciences. We give our perspective on the terminology, observation, and preservation of coherence in photophysical processes with some glimpses to the past and some looking-head to what may pave the way for scaling one of the last bastions in ultrafast science, namely, that of mode specific chemistry where it will be possible to break any specific bond by tailoring the pulse, an accomplishment that obviously would be the dream of any chemist.
相干性是超快科学中最重要的现象之一。我们从术语、观测以及光物理过程中相干性的保持等方面给出我们的观点,回顾一些过往情况,并展望可能为拓展超快科学中最后堡垒之一,即模式特异性化学铺平道路的方向。在模式特异性化学中,通过定制脉冲有可能打破任何特定的化学键,这显然是任何化学家的梦想。