Lan Chuwen, Ma He, Wang Manting, Gao Zehua, Liu Kai, Bi Ke, Zhou Ji, Xin Xiangjun
College of Applied Sciences , Beijing University of Technology , Beijing 100124 , China.
State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering , Tsinghua University , Beijing 100084 , China.
ACS Appl Mater Interfaces. 2019 Apr 17;11(15):14229-14238. doi: 10.1021/acsami.8b22466. Epub 2019 Apr 2.
Recently, all-dielectric metasurfaces (AMs) have emerged as a promising platform for high-efficiency devices ranging from the terahertz to optical ranges. However, active and fast tuning of their properties, such as amplitude, phase, and operating frequency, remains challenging. Here, a generic method is proposed for obtaining high-efficiency active AMs from the terahertz to optical ranges by using "hybrid structures" integrated with phase-change materials. Various phase-change mechanisms including metal-insulator phase change, nonvolatile phase change, and ferroelectric phase change are investigated. We first experimentally demonstrate several high-efficiency active AMs operating in the terahertz range based on hybrid structures composed of free-standing silicon microstructures covered with ultrathin phase-change nanofilms (thickness d ≪ λ). We show that both the frequencies and the strength of the Mie resonances can be efficiently tuned, resulting in unprecedented modulation depth. Furthermore, detailed analyses of available phase-change materials and their properties are provided to offer more options for active AMs. Finally, several feasible hybrid structures for active AMs in the optical range are proposed and confirmed numerically. The broad platform built in this work for active manipulation of waves from the terahertz to optical ranges may have numerous potential applications in optical devices including switches, modulators, and sensors.
近年来,全介质超表面(AMs)已成为一种有前景的平台,可用于制造从太赫兹到光学波段的高效器件。然而,对其诸如幅度、相位和工作频率等特性进行主动且快速的调谐仍然具有挑战性。在此,提出了一种通用方法,通过使用与相变材料集成的“混合结构”来获得从太赫兹到光学波段的高效主动式AMs。研究了包括金属 - 绝缘体相变、非易失性相变和铁电相变在内的各种相变机制。我们首先通过实验展示了几种基于由覆盖有超薄相变纳米薄膜(厚度d≪λ)的独立硅微结构组成的混合结构在太赫兹波段工作的高效主动式AMs。我们表明,米氏共振的频率和强度都可以得到有效调谐,从而实现前所未有的调制深度。此外,还提供了对可用相变材料及其特性的详细分析,为主动式AMs提供更多选择。最后,提出了几种用于光学波段主动式AMs的可行混合结构,并通过数值模拟进行了验证。这项工作构建的用于从太赫兹到光学波段对波进行主动操控的广阔平台,可能在包括开关、调制器和传感器在内的光学器件中具有众多潜在应用。