a National Exposure Research Laboratory , Office of Research and Development, U.S. Environmental Protection Agency , Research Triangle Park , NC , USA.
b Alion Science and Technology , Research Triangle Park , NC , USA.
J Air Waste Manag Assoc. 2019 Jun;69(6):778-788. doi: 10.1080/10962247.2019.1587553. Epub 2019 Apr 22.
Particulate matter mass (PM), trace gaseous pollutants, and select volatile organic compounds (VOCs) with meteorological variables were measured in Logan, Utah (Cache Valley), for >4 weeks during winter 2017 as part of the Utah Winter Fine Particle Study (UWFPS). Higher PM levels for short time periods and lower ozone (O) levels were present due to meteorological and mountain valley conditions. Nitrogenous pollutants were relatively strongly correlated with PM variables. Diurnal cycles of NO, O, and fine PM(PM 2.5) (aerodynamic diameter <2.5 μm [PM]) suggested formation from NO. O levels increased from early morning into midafternoon, and NO and PM increased throughout the morning, followed by sharp decreases. Toluene/benzene and xylenes/benzene ratios and VOC correlations with nitrogenous and PM species were indicative of local traffic sources. Wind sector comparisons suggested that pollutant levels were lower when winds were from nearby mountains to the east versus winds from northerly or southerly origins. : The Cache Valley in Idaho and Utah has been designated a PM nonattainment area that has been attributed to air pollution buildup during winter stagnation events. To inform state implementation plans for PM in Cache Valley and other PM nonattainment areas in Utah, a state and multiagency federal research effort known as the UWFPS was conducted in winter 2017. As part of the UWFPS, the U.S. Environmental Protection Agency (EPA) measured ground-based PM species and their precursors, VOCs, and meteorology in Logan, Utah. Results reported here from the EPA study in Logan provide additional understanding of wintertime air pollution conditions and possible sources of PM and gaseous pollutants as well as being useful for future PM control strategies in this area.
在 2017 年冬季,作为犹他冬季细颗粒物研究(UWFPS)的一部分,在美国犹他州洛根(Cache Valley)进行了超过 4 周的颗粒物质量(PM)、痕量气态污染物和部分挥发性有机化合物(VOCs)与气象变量的测量。由于气象和山谷条件,短时间内 PM 水平较高,臭氧(O)水平较低。含氮污染物与 PM 变量呈较强相关性。NO、O 和细颗粒物(PM 2.5)(空气动力学直径 <2.5μm [PM])的日变化周期表明其形成来自于 NO。O 水平从清晨升高到午后,而 NO 和 PM 在整个上午增加,随后急剧下降。甲苯/苯和二甲苯/苯的比值以及 VOC 与含氮和 PM 物质的相关性表明存在当地交通源。风区比较表明,当风从附近的山脉吹向东方时,污染物水平较低,而当风从北方或南方吹来时,污染物水平较高。
爱达荷州和犹他州的 Cache Valley 已被指定为 PM 不达标地区,这归因于冬季停滞事件期间的空气污染积聚。为了为 Cache Valley 和犹他州其他 PM 不达标的地区的 PM 州实施计划提供信息,犹他州州和多机构联邦研究机构开展了一项名为 UWFPS 的研究。作为 UWFPS 的一部分,美国环保署(EPA)在犹他州洛根测量了地面 PM 物种及其前体、VOC 和气象条件。这里报告的 EPA 洛根研究结果提供了对冬季空气污染条件以及 PM 和气态污染物可能来源的更多了解,这对于该地区未来的 PM 控制策略也很有用。