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用于能源和生物相关催化的碳纳米材料：最新进展与展望

Carbon Nanomaterials for Energy and Biorelated Catalysis: Recent Advances and Looking Forward.

作者信息

Hu Chuangang, Qu Jia, Xiao Ying, Zhao Shenlong, Chen Hao, Dai Liming

机构信息

Center of Advanced Science and Engineering for Carbon (Case4Carbon), Department of Macromolecular Science and Engineering, Case Western Reserve University (CWRU), 10900 Euclid Avenue, Cleveland, Ohio 44106, United States.

Institute of Advanced Materials for Nano-Bio Applications, School of Ophthalmology & Optometry, Wenzhou Medical University, 270 Xueyuan Xi Road, Wenzhou, Zhejiang 325027, China.

出版信息

ACS Cent Sci. 2019 Mar 27;5(3):389-408. doi: 10.1021/acscentsci.8b00714. Epub 2019 Feb 8.

DOI:10.1021/acscentsci.8b00714
PMID:30937367
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC6439526/
Abstract

Along with the wide investigation activities in developing carbon-based, metal-free catalysts to replace precious metal (e.g., Pt) catalysts for various green energy devices, carbon nanomaterials have also shown great potential for biorelated applications. This article provides a focused, critical review on the recent advances in these emerging research areas. The structure-property relationship and mechanistic understanding of recently developed carbon-based, metal-free catalysts for chemical/biocatalytic reactions will be discussed along with the challenges and perspectives in this exciting field, providing a look forward for the rational design and fabrication of new carbon-based, metal-free catalysts with high activities, remarkable selectivity, and outstanding durability for various energy-related/biocatalytic processes.

摘要

随着在开发用于各种绿色能源装置以替代贵金属（如铂）催化剂的碳基无金属催化剂方面广泛的研究活动，碳纳米材料在生物相关应用中也显示出巨大潜力。本文对这些新兴研究领域的最新进展进行了重点、批判性综述。将讨论最近开发的用于化学/生物催化反应的碳基无金属催化剂的结构-性能关系和机理理解，以及这一令人兴奋的领域中的挑战和前景，为合理设计和制备具有高活性、卓越选择性和出色耐久性的新型碳基无金属催化剂以用于各种能源相关/生物催化过程提供展望。

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