Guo Yong, Zhu Shiliu, Chen Yuxia, Li Dagang
School of Forestry and Landscape Architecture, Anhui Agricultural University, Hefei 230036, China.
College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, China.
Polymers (Basel). 2019 Jan 18;11(1):170. doi: 10.3390/polym11010170.
The damage and fracture of fiber reinforced polymer composites are vital constraints in their applications. To understand the mechanism of damage of wood fiber (WF) reinforced high density polyethylene (HDPE) composites, we used waste WF and recycled HDPE (Re-HDPE) as the raw materials and prepared high-filled WF/Re-HDPE composites via extrusion. The damage and fracture mode and failure mechanism of the composites with different WF contents (50%, 60%, and 70%) was studied under a three-point bending test by combining the acoustic emission (AE) technique and scanning electron microscope (SEM) analysis. The results show that AE technology can better assist in understanding the progress of damage and fracture process of WF/Re-HDPE composites, and determine the damage degree, damage accumulation, and damage mode. The damage and fracture process of the composites presents three main stages: the appearance of initial damage, damage accumulation, and destructive damage to fracture. The matrix deformation, fiber breakage, interface delamination, fiber-matrix debonding, fiber pull-out, and matrix cracking were the dominant modes for the damage of high-filled WF/Re-HDPE composites under bending load, and the AE signal changed in different damage stages and damage modes. In addition, the WF content and repeated loading had a significant influence on the composite's damage and fracture. The 50% and 60% WF/Re-HDPE composites produced irreversible damage when repeated load exceeded 75% of the maximum load, while 25% of the maximum load could cause irreversible damage for 70% WF/Re-HDPE composites. The damage was accumulated owing to repeated loading and the mechanical properties of the composites were seriously affected.
纤维增强聚合物复合材料的损伤与断裂是其应用中的关键制约因素。为了解木纤维(WF)增强高密度聚乙烯(HDPE)复合材料的损伤机理,我们以废弃木纤维和回收高密度聚乙烯(Re-HDPE)为原料,通过挤出工艺制备了高填充量的WF/Re-HDPE复合材料。结合声发射(AE)技术和扫描电子显微镜(SEM)分析,研究了不同木纤维含量(50%、60%和70%)的复合材料在三点弯曲试验下的损伤与断裂模式及失效机理。结果表明,AE技术能更好地辅助理解WF/Re-HDPE复合材料的损伤和断裂过程,并确定损伤程度、损伤累积情况及损伤模式。复合材料的损伤与断裂过程呈现三个主要阶段:初始损伤的出现、损伤累积以及断裂的破坏损伤。基体变形、纤维断裂、界面分层、纤维-基体脱粘、纤维拔出和基体开裂是高填充量WF/Re-HDPE复合材料在弯曲载荷下的主要损伤模式,且AE信号在不同损伤阶段和损伤模式下会发生变化。此外,木纤维含量和重复加载对复合材料的损伤与断裂有显著影响。当重复载荷超过最大载荷的75%时,50%和60%的WF/Re-HDPE复合材料会产生不可逆损伤,而对于70%的WF/Re-HDPE复合材料,最大载荷的25%即可导致不可逆损伤。由于重复加载,损伤不断累积,复合材料的力学性能受到严重影响。