Hu Yong, Lu Qiang, Chi Xiaodan, Zhang Zibo, Hu Tianyi, Li Ruijun, Yu Le, Du An
Department of Physics, College of Sciences, Northeastern University, Shenyang 110819, People's Republic of China.
Nanotechnology. 2019 Aug 9;30(32):325701. doi: 10.1088/1361-6528/ab1a57. Epub 2019 Apr 17.
In ferromagnet/antiferromagnet bilayers and core/shell nanoparticles, an exchange-bias-like loop bias phenomenon in the ferromagnet is observed solely due to the long-range dipolar interactions between ferromagnet and antiferromagnet. With increasing cooling field, the loop bias field may increase from zero in the bilayers or from a negative value in the core/shell nanoparticles to a positive saturated value, depending on the interfacial dipolar interaction and/or ferromagnetic/antiferromagnetic thickness. Using a modified Monte-Carlo method and the Meiklejohn-Bean model, the interfacial dipole fields (up to several teslas) and the domain sizes imprinted on the interfacial antiferromagnet are explicitly calculated to elucidate the cooling field dependence of loop bias, which is governed by distinct mechanisms at the flat and curved interfaces. Finally, through simply discussing the roles of lattice structure, ferromagnetic dipolar interaction, and simulation time, it is evidenced that the dipole-induced loop bias is ubiquitous and applicable for stabilizing a ferromagnet, irrespective of the interface mismatch and the undeterministic diffusion between different ingredients. This work helps us to develop the spintronic devices with nonatomic-contact nanostructure assemblies.
在铁磁体/反铁磁体双层结构以及核壳纳米颗粒中,仅由于铁磁体与反铁磁体之间的长程偶极相互作用,就会在铁磁体中观察到类似交换偏置的环路偏置现象。随着冷却场的增加,环路偏置场可能从双层结构中的零值或核壳纳米颗粒中的负值增加到正的饱和值,这取决于界面偶极相互作用和/或铁磁体/反铁磁体的厚度。使用改进的蒙特卡罗方法和梅克莱约翰 - 比恩模型,明确计算了界面偶极场(高达几特斯拉)以及印刻在界面反铁磁体上的畴尺寸,以阐明环路偏置对冷却场的依赖性,这在平面和弯曲界面处由不同机制控制。最后,通过简单讨论晶格结构、铁磁偶极相互作用和模拟时间的作用,证明了偶极诱导的环路偏置是普遍存在的,并且适用于稳定铁磁体,而与界面失配以及不同成分之间不确定的扩散无关。这项工作有助于我们开发具有非原子接触纳米结构组件的自旋电子器件。