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[利用杭州地区地基太阳光度计测量确定的柱积分气溶胶光学特性]

[Column-integrated Aerosol Optical Properties Determined Using Ground-based Sun Photometry Measurements in the Hangzhou Region].

作者信息

Qi Bing, Che Hui-Zheng, Xu Ting-Ting, Du Rong-Guang, Hu De-Yun, Liang Zhuo-Ran, Ma Qian-Li, Yao Jie

机构信息

Hangzhou Meteorological Bureau, Hangzhou 310051, China.

Key Laboratory of Atmospheric Chemistry, China Meteorological Administration, Beijing 100081, China.

出版信息

Huan Jing Ke Xue. 2019 Apr 8;40(4):1604-1612. doi: 10.13227/j.hjkx.201808071.

DOI:10.13227/j.hjkx.201808071
PMID:31087900
Abstract

To investigate the optical properties of aerosols in the Hangzhou region (Hangzhou, Tonglu, Jiande, and Chun'an), the aerosol optical depth (AOD), Ångström exponent (AE), single scattering albedo (SSA), and aerosol size distribution (ASD) were measured using CIMEL sun-photometers in 2012. The results showed that the annual average values of AOD in Hangzhou, Tonglu, Jiande, and Chun'an were 0.94±0.16, 0.84±0.17, 0.82±0.22, and 0.71±0.20, respectively. The values generally decreased from the northeast to the southwest, and represented one of highest AOD districts in the Yangtze River Delta, China. The annual average values of AE were 1.24±0.12, 1.19±0.17, 1.06±0.04, and 1.04±0.10, respectively, indicating that particles with small average effective radii were predominant. The relatively lower AE values in March and April were generally attributed to the long-range transport of dust aerosols from Northwest China. Obvious diurnal variations in the AOD were found in Hangzhou, Tonglu, and Jiande, but not in Chun'an. An average fine-mode effective radius of0.15 μm was observed in spring, autumn, and winter, while a value of0.25 μm was observed in summer, in conjunction with aerosol hygroscopic growth. An average coarse-mode effective radius of~2.94 μm was observed in summer, autumn, and winter, which was higher than the value in spring. The annual average values of SSA were 0.91±0.01, 0.92±0.03, 0.92±0.02, 0.93±0.02, respectively, indicating that the particles had relatively strong to moderate absorption. Characterization of the aerosol types showed the predominance of biomass burning and urban industrial type aerosols in Hangzhou, while mixed type aerosols were observed in Tonglu, Jiande, and Chun'an.

摘要

为研究杭州地区(杭州、桐庐、建德和淳安)气溶胶的光学特性,2012年使用CIMEL太阳光度计测量了气溶胶光学厚度(AOD)、Ångström指数(AE)、单次散射反照率(SSA)和气溶胶粒径分布(ASD)。结果表明,杭州、桐庐、建德和淳安的AOD年平均值分别为0.94±0.16、0.84±0.17、0.82±0.22和0.71±0.20。这些值总体上从东北向西南递减,代表了中国长江三角洲地区AOD最高的区域之一。AE的年平均值分别为1.24±0.12、1.19±0.17、1.06±0.04和1.04±0.10,表明平均有效半径较小的颗粒占主导。3月和4月相对较低的AE值通常归因于来自中国西北地区沙尘气溶胶的远距离传输。在杭州、桐庐和建德发现了AOD明显的日变化,但在淳安未发现。在春季、秋季和冬季观测到平均细模态有效半径约为0.15μm,而在夏季观测到的值约为0.25μm,同时伴有气溶胶吸湿增长。在夏季、秋季和冬季观测到平均粗模态有效半径约为2.94μm,高于春季的值。SSA的年平均值分别为0.91±0.01、0.92±0.03、0.92±0.02、0.93±0.02,表明颗粒具有相对较强到中等的吸收能力。气溶胶类型特征表明,杭州以生物质燃烧和城市工业型气溶胶为主,而桐庐、建德和淳安观测到的是混合型气溶胶。

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