Burdin Sébastien, Lacroix Claudine
Université de Bordeaux, CNRS, LOMA, UMR 5798, 33400 Talence, France.
J Phys Condens Matter. 2019 Oct 2;31(39):395601. doi: 10.1088/1361-648X/ab2701. Epub 2019 Jun 4.
We study the low energy states of the Kondo alloy model (KAM) as function of the magnetic impurity concentration per site, x, and the conduction electron average site occupation, n . In previous works, two different Fermi liquid regimes had been identified at strong Kondo coupling [Formula: see text], that may be separated by a transition at x = n . Here, we analyze the KAM for finite [Formula: see text] on a Bethe lattice structure. First, using the mean-field coherent potential approximation (DMFT-CPA) which is exact at lattice coordination [Formula: see text], we show that the real part of the local potential scattering may be located outside the conduction electron band, revealing a possible breakdown of Luttinger theorem for intermediate values of impurity concentration x. Unusual physical signatures are expected, e.g. in ARPES experiments. In order to take into account fluctuations associated with finite dimensionality, i.e. finite Z, we extend this analysis by studying the KAM with an adaptation of the statistical-DMFT method that was developped elsewhere. We review the distributions of local potential scattering and their evolution with model parameters: concentration, strength of Kondo coupling, coordination number, local site neighborhood, connection with percolation issue. Relevence for Kondo alloys material with f -electrons is also discussed.
我们研究了近藤合金模型(KAM)的低能态,它是每个格点上磁性杂质浓度(x)以及传导电子平均格点占据数(n)的函数。在之前的工作中,在强近藤耦合([公式:见正文])下确定了两种不同的费米液体 regime,它们可能在(x = n)处的转变中被分开。在这里,我们在贝特晶格结构上分析有限([公式:见正文])的KAM。首先,使用在晶格配位数([公式:见正文])处精确的平均场相干势近似(DMFT - CPA),我们表明局部势散射的实部可能位于传导电子能带之外,这揭示了对于杂质浓度(x)的中间值,卢廷格定理可能失效。预计会有不寻常的物理特征,例如在角分辨光电子能谱(ARPES)实验中。为了考虑与有限维数相关的涨落,即有限的(Z),我们通过用在其他地方发展的统计DMFT方法的一种改编来研究KAM,从而扩展了这一分析。我们回顾了局部势散射的分布及其随模型参数的演化:浓度、近藤耦合强度、配位数、局部格点邻域、与渗流问题的联系。还讨论了与具有(f)电子的近藤合金材料的相关性。