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大气颗粒物结合态汞的测量与分布:综述

Measurements and Distribution of Atmospheric Particulate-Bound Mercury: A Review.

作者信息

Zhang Hui, Fu Xuewu, Wang Xun, Feng Xinbin

机构信息

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang, 550002, China.

CAS Center for Excellence in Quaternary Science and Global Change, Xi'an, 710061, China.

出版信息

Bull Environ Contam Toxicol. 2019 Jul;103(1):48-54. doi: 10.1007/s00128-019-02663-5. Epub 2019 Jun 24.

Abstract

Atmospheric particulate-bound mercury (PBM) plays an important role in the geochemical cycling of mercury (Hg). This study reviewed research progress of the PBM, including the possible emission and deposition pathways, measurement methods and the global distribution. The primary PBM sources are anthropogenic sources, but natural sources could be also a considerable contributor, for instance, chemical transport and dust in the arid and desert area. Different filter methods, such as quartz fibre filters, have been applied to the PBM measurement, and PBM can also be real-time monitored automatically. Generally, the average PBM concentrations were higher in the Northern Hemisphere than in the Southern Hemisphere. However, the PBM level of Antarctica is quite high. PBM concentrations were higher in the urban areas than in the remote areas, and there was a high PBM level in the developing countries. Moreover, high PBM concentrations were observed in the range 20°-60° of northern latitude.

摘要

大气颗粒物结合态汞(PBM)在汞(Hg)的地球化学循环中起着重要作用。本研究综述了PBM的研究进展,包括其可能的排放和沉降途径、测量方法以及全球分布情况。PBM的主要来源是人为源,但自然源也可能是一个相当重要的贡献者,例如干旱和沙漠地区的化学传输和沙尘。不同的过滤方法,如石英纤维滤膜,已应用于PBM的测量,并且PBM也可以进行自动实时监测。一般来说,北半球的PBM平均浓度高于南半球。然而南极地区的PBM水平相当高。城市地区的PBM浓度高于偏远地区,并且发展中国家存在较高的PBM水平。此外,在北纬20°-60°范围内观测到较高的PBM浓度。

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