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绝缘体热扩散率的下限。

A lower bound to the thermal diffusivity of insulators.

作者信息

Behnia Kamran, Kapitulnik Aharon

机构信息

Laboratoire Physique et Etude de Matériaux (CNRS-Sorbonne Université), ESPCI Paris, PSL Research University, 75005 Paris, France. II. Physikalisches Institut, Universität zu Köln, 50937 Köln, Germany.

出版信息

J Phys Condens Matter. 2019 Oct 9;31(40):405702. doi: 10.1088/1361-648X/ab2db6. Epub 2019 Jun 28.

Abstract

It has been known for decades that thermal conductivity of insulating crystals becomes proportional to the inverse of temperature when the latter is comparable to, or higher than, the Debye temperature. This behavior has been understood as resulting from Umklapp scattering among phonons. We put under scrutiny the magnitude of the thermal diffusion constant in this regime and find that it does not fall below a threshold set by the square of sound velocity times the Planckian time ([Formula: see text]). The conclusion, based on scrutinizing the ratio in cubic crystals with high thermal resistivity, appears to hold even in glasses where Umklapp events are not conceivable. Explaining this boundary, reminiscent of a recently-noticed limit for charge transport in metals, is a challenge to theory.

摘要

几十年来,人们已经知道,当温度与德拜温度相当或高于德拜温度时,绝缘晶体的热导率与温度的倒数成正比。这种行为被理解为声子之间的倒逆散射所致。我们仔细研究了该区域内热扩散常数的大小,发现它不会低于声速平方乘以普朗克时间所设定的阈值([公式:见正文])。基于对具有高热阻率的立方晶体中该比率的仔细研究得出的这一结论,似乎在无法想象倒逆事件的玻璃中也成立。解释这个边界,让人想起最近在金属中发现的电荷输运极限,这对理论来说是一个挑战。

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