Luo Dongxiang, Chen Qizan, Qiu Ying, Zhang Menglong, Liu Baiquan
School of Materials and Energy, Guangdong University of Technology, Guangzhou 510006, China.
Guangdong R&D Center for Technological Economy, Guangzhou 510000, China.
Nanomaterials (Basel). 2019 Jul 12;9(7):1007. doi: 10.3390/nano9071007.
Recently, all-inorganic perovskite light-emitting diodes (PeLEDs) have attracted both academic and industrial interest thanks to their outstanding properties, such as high efficiency, bright luminance, excellent color purity, low cost and potentially good operational stability. Apart from the design and treatment of all-inorganic emitters, the device engineering is another significant factor to guarantee the high performance. In this review, we have summarized the state-of-the-art concepts for device engineering in all-inorganic PeLEDs, where the charge injection, transport, balance and leakage play a critical role in the performance. First, we have described the fundamental concepts of all-inorganic PeLEDs. Then, we have introduced the enhancement of device engineering in all-inorganic PeLEDs. Particularly, we have comprehensively highlighted the emergence of all-inorganic PeLEDs, strategies to improve the hole injection, approaches to enhance the electron injection, schemes to increase the charge balance and methods to decrease the charge leakage. Finally, we have clarified the issues and ways to further enhance the performance of all-inorganic PeLEDs.
最近,全无机钙钛矿发光二极管(PeLEDs)因其出色的性能,如高效率、高亮度、优异的色纯度、低成本以及潜在的良好运行稳定性,而引起了学术界和工业界的关注。除了全无机发光体的设计和处理外,器件工程是保证高性能的另一个重要因素。在这篇综述中,我们总结了全无机PeLEDs器件工程的最新概念,其中电荷注入、传输、平衡和泄漏对性能起着关键作用。首先,我们描述了全无机PeLEDs的基本概念。然后,我们介绍了全无机PeLEDs器件工程的增强。特别是,我们全面强调了全无机PeLEDs的出现、改善空穴注入的策略、增强电子注入的方法、增加电荷平衡的方案以及减少电荷泄漏的方法。最后,我们阐明了进一步提高全无机PeLEDs性能的问题和方法。