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中国城市土壤中的多环芳烃:分布、影响因素、健康风险和回归预测。

Polycyclic aromatic hydrocarbons in urban soils of China: Distribution, influencing factors, health risk and regression prediction.

机构信息

Institute of Environmental Engineering, School of Metallurgy and Environment, Central South University, Changsha, 410083, People's Republic of China.

Institute of Environmental Engineering, School of Metallurgy and Environment, Central South University, Changsha, 410083, People's Republic of China.

出版信息

Environ Pollut. 2019 Nov;254(Pt A):112930. doi: 10.1016/j.envpol.2019.07.098. Epub 2019 Jul 20.

Abstract

Polycyclic aromatic hydrocarbons (PAHs) in urban soils are a risk to the health of residents. To predict those risks, the distribution and the factors influencing the concentration of PAHs were studied by collecting 1120 records of soil PAHs published during 2006-2017 from 26 cities. The mean concentrations of 16 PAHs (∑PAHs) in soil varied from 123 μg/kg to 5568 μg/kg, with a mean value of 1083 μg/kg, suggesting that a few cities were polluted. The distribution of ∑PAHs in the cities followed two gradients, namely from northern China through eastern China to southern China and from industrial cities through developed cities to cities that are main tourist attractions. The concentrations were significantly correlated to annual temperature, the efficiency of energy use, and to such measures of air quality as PM and NO concentrations. A regression equation developed to predict the concentration of ∑PAHs in soil and the corresponding health risks to residents of 35 major Chinese cities of China showed that the risks to adults and children were slight in most cities but those in a few industrial cities were of concern, and field investigations are recommended to assess the risk in greater detail. The method offers a useful tool for predicting such risks in other cities even when data on soils PAHs are not available.

摘要

多环芳烃(PAHs)在城市土壤中对居民的健康构成威胁。为了预测这些风险,收集了 2006-2017 年 26 个城市发表的 1120 份土壤多环芳烃记录,研究了其分布和影响浓度的因素。土壤中 16 种多环芳烃(∑PAHs)的平均浓度为 123μg/kg 至 5568μg/kg,平均值为 1083μg/kg,表明有少数城市受到污染。∑PAHs 在城市中的分布遵循两个梯度,即从中国北方经华东到华南,从工业城市经发达城市到主要旅游城市。浓度与年平均温度、能源利用效率以及 PM 和 NO 浓度等空气质量指标显著相关。建立了一个回归方程来预测土壤中∑PAHs 的浓度以及对中国 35 个主要城市居民的相应健康风险,结果表明,大多数城市的成年人和儿童的风险较小,但少数工业城市的风险值得关注,建议进行实地调查以更详细地评估风险。该方法为预测其他城市的此类风险提供了有用的工具,即使没有土壤多环芳烃的数据。

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