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通过直接测量范霍夫分布函数的时间积分的跑动,从弹性中子散射中获得动力学信息。

Dynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van Hove distribution function.

机构信息

School of Physics, University College Dublin, Dublin 4, Ireland.

School of Chemistry, University College Dublin, Dublin 4, Ireland.

出版信息

Sci Rep. 2019 Aug 2;9(1):11284. doi: 10.1038/s41598-019-46835-z.

Abstract

We present a new neutron-scattering approach to access the van Hove distribution function directly in the time domain, I(t), which reflects the system dynamics. Currently, I(t) is essentially determined from neutron energy-exchange. Our method consists of the straightforward measurement of the running time-integral of I(t), by computing the portion of scattered neutrons corresponding to species at rest within a time t, (conceptually elastic scattering). Previous attempts failed to recognise this connection. Starting from a theoretical standpoint, a practical realisation is assessed via numerical methods and an instrument simulation.

摘要

我们提出了一种新的中子散射方法,可直接在时域中获取范霍夫分布函数 I(t),从而反映系统动态。目前,I(t)主要通过中子能量交换来确定。我们的方法包括通过计算在时间 t 内对应于静止物质的散射中子部分,直接测量 I(t)的积分,(概念上是弹性散射)。之前的尝试未能认识到这种联系。从理论角度出发,通过数值方法和仪器模拟来评估实际实现。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3148/6677729/af18d2f1b77a/41598_2019_46835_Fig1_HTML.jpg

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