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室内颗粒物测量:指标、传感器、需求和应用综述。

Particulate Matter Measurement Indoors: A Review of Metrics, Sensors, Needs, and Applications.

机构信息

Lancaster Environment Centre , Lancaster University , Lancaster LA1 4YQ , United Kingdom.

State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry , Chinese Academy of Sciences , 511 Kehua Rd , Tianhe, Guangzhou 510640 , China.

出版信息

Environ Sci Technol. 2019 Oct 15;53(20):11644-11656. doi: 10.1021/acs.est.9b03425. Epub 2019 Sep 25.

Abstract

Many populations spend ∼90% of their time indoors, with household particulate matter being linked to millions of premature deaths worldwide. Particulate matter is currently measured using particle mass, particle number, and particle size distribution metrics, with other metrics, such as particle surface area, likely to be of increasing importance in the future. Particulate mass is measured using gravimetric methods, tapered element oscillating microbalances, and beta attenuation instruments and is best suited to use in compliance monitoring, trend analysis, and high spatial resolution measurements. Particle number concentration is measured by condensation particle counters, optical particle counters, and diffusion chargers. Particle number measurements are best suited to source characterization, trend analysis and ultrafine particle investigations. Particle size distributions are measured by gravimetric impactors, scanning mobility particle sizers, aerodynamic particle sizers, and fast mobility particle sizers. Particle size distribution measurements are most useful in source characterization and particulate matter property investigations, but most measurement options remain expensive and intrusive. However, we are on the cusp of a revolution in indoor air quality monitoring and management. Low-cost sensors have potential to facilitate personalized information about indoor air quality (IAQ), allowing citizens to reduce exposures to PM indoors and to resolve potential dichotomies between promoting healthy IAQ and energy efficient buildings. Indeed, the low cost will put this simple technology in the hands of citizens who wish to monitor their own IAQ in the home or workplace, to inform lifestyle decisions. Low-cost sensor networks also look promising as the solution to measuring spatial distributions of PM indoors, however, there are important sensor/data quality, technological, and ethical barriers to address with this technology. An improved understanding of epidemiology is essential to identify which metrics correlate most with health effects, allowing indoor specific PM standards to be developed and to inform the future of experimental applications.

摘要

许多人在室内度过了大约 90%的时间,而家庭颗粒物与全球数百万人的过早死亡有关。颗粒物目前使用颗粒物质量、颗粒物数量和颗粒物粒径分布指标进行测量,而其他指标(如颗粒物表面积)在未来可能变得越来越重要。颗粒物质量使用重量法、锥形元件振荡微天平(tapered element oscillating microbalances)和β衰减仪器进行测量,最适合用于合规监测、趋势分析和高空间分辨率测量。颗粒数浓度通过凝结核计数器、光学粒子计数器和扩散充电器进行测量。颗粒数测量最适合用于源特征描述、趋势分析和超细颗粒研究。粒径分布通过重量撞击器、扫描迁移率颗粒计数器、空气动力学颗粒计数器和快速迁移率颗粒计数器进行测量。粒径分布测量最有利于源特征描述和颗粒物特性研究,但大多数测量选项仍然昂贵且具有侵入性。然而,我们正处于室内空气质量监测和管理的革命的边缘。低成本传感器有可能促进室内空气质量(IAQ)的个性化信息,使公民能够减少在室内接触 PM 的机会,并解决促进健康的 IAQ 和节能建筑之间可能存在的二分法。事实上,低成本将使这项简单的技术掌握在希望在家中或工作场所监测自己室内空气质量的公民手中,以做出生活方式决策。低成本传感器网络也有望成为测量室内 PM 空间分布的解决方案,然而,这项技术还存在着重要的传感器/数据质量、技术和伦理障碍需要解决。改善对流行病学的理解对于确定与健康影响最相关的指标至关重要,这将有助于制定针对室内特定 PM 的标准,并为未来的实验应用提供信息。

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