Paterson Gary W, Lamb Raymond J, Ballabriga Rafael, Maneuski Dima, O'Shea Val, McGrouther Damien
SUPA, School of Physics and Astronomy, University of Glasgow, Glasgow G12 8QQ, United Kingdom.
CERN, 1211 Geneva Geneva, 23, Switzerland.
Ultramicroscopy. 2020 Mar;210:112917. doi: 10.1016/j.ultramic.2019.112917. Epub 2019 Dec 7.
Detector developments are currently enabling new capabilities in the field of transmission electron microscopy (TEM). We have investigated the limits of a hybrid pixel detector, Medipix3, to record dynamic, time varying, electron signals. Operating with an energy of 60 keV, we have utilised electrostatic deflection to oscillate electron beam position on the detector. Adopting a pump-probe imaging strategy, we have demonstrated that temporal resolutions three orders of magnitude smaller than are available for typically used TEM imaging detectors are possible. Our experiments have shown that energy deposition of the primary electrons in the hybrid pixel detector limits the overall temporal resolution. Through adjustment of user specifiable thresholds or the use of charge summing mode, we have obtained images composed from summing 10,000s frames containing single electron events to achieve temporal resolution less than 100 ns. We propose that this capability can be directly applied to studying repeatable material dynamic processes but also to implement low-dose imaging schemes in scanning transmission electron microscopy.
探测器的发展目前正在为透射电子显微镜(TEM)领域带来新的功能。我们研究了混合像素探测器Medipix3记录动态、随时间变化的电子信号的极限。在60 keV的能量下运行,我们利用静电偏转使电子束在探测器上的位置振荡。采用泵浦-探测成像策略,我们已经证明,与通常使用的TEM成像探测器相比,时间分辨率可以小三个数量级。我们的实验表明,初级电子在混合像素探测器中的能量沉积限制了整体时间分辨率。通过调整用户可指定的阈值或使用电荷求和模式,我们获得了由包含单电子事件的10000帧求和组成的图像,以实现小于100 ns的时间分辨率。我们认为,这种能力不仅可以直接应用于研究可重复的材料动态过程,还可以应用于在扫描透射电子显微镜中实施低剂量成像方案。