Coexistence of the Kondo effect and spin glass physics in Fe-doped NbS.

We report the coexistence of the Kondo effect and spin glass behavior in Fe-doped NbS single crystals. The Fe NbS shows the resistance minimum and negative magnetoresistance due to the Kondo effect, and exhibits no superconducting behavior at low temperatures. The resistance curve follows a numerical renormalization-group theory using the Kondo temperature [Formula: see text] K for x  =  0.01 as evidence of Kondo effect. Scanning tunneling microscope/spectroscopy (STM/STS) revealed the presence of Fe atoms near sulfur atoms and asymmetric spectra. The magnetic susceptibility exhibits a feature of spin glass. The static critical exponents determined by the universal scaling of the nonlinear part of the susceptibility suggest a three-dimensional Heisenberg spin glass. The doped-Fe atoms in the intra- and inter-layers revealed by the x-ray result can realize the coexistence of the Kondo effect and spin glass.