Chemistry Department, Lomonosov Moscow State University, 119991 Moscow, Russia.
Department of Biochemistry and Molecular Pharmacology, University of Massachusetts Medical School, Worcester, MA 01655, USA.
Biomolecules. 2019 Dec 18;10(1):8. doi: 10.3390/biom10010008.
In mammals, DNA methylation is necessary for the maintenance of genomic stability, gene expression regulation, and other processes. During malignant diseases progression, changes in both DNA methylation patterns and DNA methyltransferase (MTase) genes are observed. Human de novo MTase DNMT3A is most frequently mutated in acute myeloid leukemia (AML) with a striking prevalence of R882H mutation, which has been extensively studied. Here, we investigate the functional role of the missense mutations (S714C, R635W, R736H, R771L, P777R, and F752V) found in the catalytic domain of DNMT3A in AML patients. These were accordingly mutated in the murine Dnmt3a catalytic domain (S124C, R45W, R146H, R181L, P187R, and F162V) and in addition, one-site CpG-containing DNA substrates were used as a model system. The 3-15-fold decrease (S124C and P187R) or complete loss (F162V, R45W, and R146H) of Dnmt3a-CD methylation activity was observed. Remarkably, Pro 187 and Arg 146 are not located at or near the Dnmt3a functional motives. Regulatory protein Dnmt3L did not enhance the methylation activity of R45W, R146H, P187R, and F162V mutants. The key steps of the Dnmt3a-mediated methylation mechanism, including DNA binding and transient covalent intermediate formation, were examined. There was a complete loss of DNA-binding affinity for R45W located in the AdoMet binding region and for R146H. Dnmt3a mutants studied in vitro suggest functional impairment of DNMT3A during pathogenesis.
在哺乳动物中,DNA 甲基化对于维持基因组稳定性、基因表达调控和其他过程是必要的。在恶性疾病进展过程中,观察到 DNA 甲基化模式和 DNA 甲基转移酶(MTase)基因的变化。人类从头甲基转移酶 DNMT3A 在急性髓细胞白血病(AML)中最常发生突变,其中 R882H 突变的发生率很高,已被广泛研究。在这里,我们研究了在 AML 患者中发现的 DNMT3A 催化结构域中的错义突变(S714C、R635W、R736H、R771L、P777R 和 F752V)的功能作用。这些突变相应地发生在鼠 Dnmt3a 催化结构域中(S124C、R45W、R146H、R181L、P187R 和 F162V),此外,还使用单一位点 CpG 含有 DNA 底物作为模型系统。观察到 Dnmt3a-CD 甲基化活性降低了 3-15 倍(S124C 和 P187R)或完全丧失(F162V、R45W 和 R146H)。值得注意的是,脯氨酸 187 和精氨酸 146 不位于或靠近 Dnmt3a 功能基序。调节蛋白 Dnmt3L 并没有增强 R45W、R146H、P187R 和 F162V 突变体的甲基化活性。检查了 Dnmt3a 介导的甲基化机制的关键步骤,包括 DNA 结合和瞬时共价中间产物的形成。位于 AdoMet 结合区域的 R45W 和 R146H 的 DNA 结合亲和力完全丧失。在体外研究的 Dnmt3a 突变体表明,DNMT3A 在发病机制中功能受损。