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具有正介电各向异性的向列型液晶中脐点产生的理论预测。

Theoretical Prediction of Umbilics Creation in Nematic Liquid Crystals with Positive Dielectric Anisotropy.

作者信息

Habibpourmoghadam Atefeh

机构信息

Department of Chemistry, Paderborn University, Warburger Straße 100, 33098 Paderborn, Germany.

出版信息

ACS Omega. 2019 Dec 5;4(25):21459-21468. doi: 10.1021/acsomega.9b03158. eCollection 2019 Dec 17.

Abstract

Optically assisted electrical generation of umbilic defects, arising in homeotropically aligned nematic liquid crystal cells and known as topological templates for the generation of optical vortices, are reported in nematic liquid crystals with positive dielectric anisotropy in detail. It is shown that nematic liquid crystals with positive dielectric anisotropy can serve as a stable and efficient medium for the optical vortex generation from both linearly and circularly polarized input Gaussian beams. Hybrid cells made from a thin layer of nematic liquid crystal confined between a photoresponsive slab of iron-doped lithium niobate and a glass plate coated with an active material, i.e., indium tin oxide, were studied. Exposure to a laser beam locally induces a photovoltaic field in the iron-doped lithium niobate substrate, which can penetrate into the liquid crystal film and induce realignment of molecules. The photovoltaic field drives charge carrier accumulation at the interface of indium tin oxide with the liquid crystal, which effectively modifies the shape and symmetry of the electric field. The photovoltaic field has a continuous radial distribution in the transverse -plane, weakening with increasing distance from the light irradiation center, where the electric field is normal to the cell plane. Umbilics are created as a result of the liquid crystal tendency to realign parallel to the electric field. Numerical studies of the transmitted intensity profiles in between linear polarizers reveal optical vortex pattern (of four and eight brushes) characteristics for the umbilical defects. The application of crossed circular polarizers results in annular-shaped intensity patterns as a result of spin-to-orbital angular momentum conversions, which give rise to the optical vortices.

摘要

详细报道了在垂直排列的向列型液晶盒中产生的光学辅助电致脐点缺陷,这种缺陷被称为产生光学涡旋的拓扑模板,该研究针对具有正介电各向异性的向列型液晶展开。研究表明,具有正介电各向异性的向列型液晶可作为一种稳定且高效的介质,用于从线偏振和圆偏振输入高斯光束中产生光学涡旋。研究了由一层薄的向列型液晶制成的混合盒,该液晶层被限制在掺铁铌酸锂的光响应平板和涂有活性材料(即氧化铟锡)的玻璃板之间。激光束照射会在掺铁铌酸锂衬底中局部感应出一个光伏场,该光伏场可穿透到液晶膜中并诱导分子重新排列。光伏场驱动电荷载流子在氧化铟锡与液晶的界面处积累,这有效地改变了电场的形状和对称性。光伏场在横向平面上具有连续的径向分布,随着距光照射中心距离的增加而减弱,在该中心处电场垂直于盒平面。由于液晶倾向于与电场平行重新排列,从而产生了脐点。线性偏振器之间透射强度分布的数值研究揭示了脐点缺陷的光学涡旋图案(四刷和八刷)特征。交叉圆偏振器的应用由于自旋到轨道角动量的转换而导致环形强度图案,从而产生光学涡旋。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b003/6921641/27e83bbc32a9/ao9b03158_0010.jpg

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