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2015 年厄尔尼诺现象期间亚马逊地区大都市的生物质燃烧影响:一氧化碳和左旋葡聚糖浓度的增加。

Impact of biomass burning on a metropolitan area in the Amazon during the 2015 El Niño: The enhancement of carbon monoxide and levoglucosan concentrations.

机构信息

Postgraduate Program in Climate and Environment (CLIAMB, INPA/UEA), Av. André Araújo, 2936, Campus II, Aleixo, 69060-001, Manaus, Amazonas, Brazil.

Federal University of Amazonas, Department of Chemistry, Av. General Rodrigo Octavio Jordão Ramos, 1200 - Coroado I, 69067-005, Manaus, Amazonas, Brazil.

出版信息

Environ Pollut. 2020 May;260:114029. doi: 10.1016/j.envpol.2020.114029. Epub 2020 Jan 22.

Abstract

Extreme droughts associated with changes in the climate have occurred every 5 years in the Amazon during the 21st century, with the most severe being in 2015. The increase in biomass burning (BB) events that occurred during the 2015 drought had several negative socioeconomic and environmental impacts, one of which was a decrease in the air quality. This study is an investigation into the air quality in the Manaus Metropolitan Region (MMR) (central Amazon, Brazil) during the dry (September to October) and wet (April to May) seasons of 2015 and 2016. A strong El Niño event began during the wet season of 2015 and ended during the wet season of 2016. Particulate matter samples were collected in the MMR during 2015 and 2016, and analyses of the satellite-estimated total carbon monoxide (CO) column and observed levoglucosan concentrations were carried out. Levoglucosan has been shown to be significantly correlated with regional fires and is a well-established chemical tracer for the atmospheric particulates emitted by BB, and CO can be treated as a gaseous-phase tracer for BB. The number of BB events increased significantly during the El Niño period when compared to the average number during 2003-2016. Consequently, the total CO column and levoglucosan concentration values in the MMR increased by 15% and 500%, respectively, when compared to the normal conditions. These results indicate that during the period that was analyzed, the impacts of BB were exacerbated during the strong El Niño event as compared to the non-El Niño period. In this study, we provided evidence that the air quality in the MMR will degrade in the future if droughts and BB occurrences continue to increase.

摘要

21 世纪,亚马逊地区每 5 年就会发生一次与气候变化相关的极端干旱,其中最严重的一次发生在 2015 年。2015 年干旱期间,生物质燃烧(BB)事件的增加对社会经济和环境产生了诸多负面影响,其中之一是空气质量下降。本研究调查了 2015 年和 2016 年干季(9 月至 10 月)和湿季(4 月至 5 月)马瑙斯大都市区(MMR)(巴西亚马逊中心)的空气质量。2015 年湿季开始出现强烈厄尔尼诺现象,并持续到 2016 年湿季结束。在 2015 年和 2016 年,在 MMR 收集了颗粒物样本,并对卫星估计的总一氧化碳(CO)柱和观测到的左旋葡聚糖浓度进行了分析。左旋葡聚糖已被证明与区域火灾显著相关,是 BB 排放的大气颗粒物的成熟化学示踪剂,而 CO 可以作为 BB 的气相示踪剂。与 2003-2016 年的平均值相比,厄尔尼诺期间 BB 事件的数量显著增加。因此,与正常情况相比,MMR 的总 CO 柱和左旋葡聚糖浓度值分别增加了 15%和 500%。这些结果表明,在所分析的时间段内,与非厄尔尼诺期间相比,强厄尔尼诺事件使 BB 的影响加剧。在本研究中,我们提供的证据表明,如果干旱和 BB 事件继续增加,未来 MMR 的空气质量将会恶化。

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