Benedek Giorgio, Miret-Artés Salvador, Manson J R, Ruckhofer Adrian, Ernst Wolfgang E, Tamtögl Anton
Donostia International Physics Center (DIPC), Paseo Manuel de Lardizabal, 4, 20018 Donostia-San Sebastian, Spain.
Dipartimento di Scienza dei Materiali, Università di Milano-Bicocca, Via Cozzi 53, 20125 Milano, Italy.
J Phys Chem Lett. 2020 Mar 5;11(5):1927-1933. doi: 10.1021/acs.jpclett.9b03829. Epub 2020 Feb 24.
He atom scattering has been demonstrated to be a sensitive probe of the electron-phonon interaction parameter λ at metal and metal-overlayer surfaces. Here it is shown that the theory linking λ to the thermal attenuation of atom scattering spectra (the Debye-Waller factor) can be applied to topological semimetal surfaces, such as the quasi-one-dimensional charge-density-wave system Bi(114) and the layered pnictogen chalcogenides. The electron-phonon coupling, as determined for several topological insulators belonging to the class of bismuth chalcogenides, suggests a dominant contribution of the surface quantum well states over the Dirac electrons in terms of λ.
氦原子散射已被证明是探测金属及金属覆盖层表面电子 - 声子相互作用参数λ的灵敏探针。本文表明,将λ与原子散射光谱的热衰减(德拜 - 瓦勒因子)联系起来的理论可应用于拓扑半金属表面,如准一维电荷密度波系统Bi(114)和层状氮族硫族化合物。对于几种属于铋硫族化合物类别的拓扑绝缘体所确定的电子 - 声子耦合表明,就λ而言,表面量子阱态比狄拉克电子起主要作用。