Ruckhofer Adrian, Benedek Giorgio, Bremholm Martin, Ernst Wolfgang E, Tamtögl Anton
Institute of Experimental Physics, Graz University of Technology, Petersgasse 16, 8010 Graz, Austria.
Dipartimento di Scienza dei Materiali, Università degli Studi di Milano-Bicocca, Via R. Cozzi 55, 20125 Milano, Italy.
Nanomaterials (Basel). 2023 Jan 24;13(3):476. doi: 10.3390/nano13030476.
While parallel segments in the Fermi level contours, often found at the surfaces of topological insulators (TIs), would imply "strong" nesting conditions, the existence of charge-density waves (CDWs)-periodic modulations of the electron density-has not been verified up to now. Here, we report the observation of a CDW at the surface of the TI Bi2Te2Se(111), below ≈350K, by helium-atom scattering and, thus, experimental evidence for a CDW involving Dirac topological electrons. Deviations of the order parameter observed below 180K, and a low-temperature break of time reversal symmetry, suggest the onset of a spin-density wave with the same period as the CDW in the presence of a prominent electron-phonon interaction, originating from Rashba spin-orbit coupling.
虽然在拓扑绝缘体(TI)表面经常发现的费米能级轮廓中的平行线段意味着“强”嵌套条件,但迄今为止,电荷密度波(CDW)——电子密度的周期性调制——的存在尚未得到证实。在这里,我们报告了通过氦原子散射在TI Bi2Te2Se(111)表面低于约350K时观察到的CDW,从而获得了涉及狄拉克拓扑电子的CDW的实验证据。在180K以下观察到的序参量偏差以及时间反演对称性的低温破坏,表明在存在源于Rashba自旋轨道耦合的显著电子-声子相互作用的情况下,出现了与CDW具有相同周期的自旋密度波。