Banerjee Abhisek, Saveliev Alexei
Department of Mechanical and Aerospace Engineering, North Carolina State University, Raleigh, NC, United States.
Front Chem. 2020 Feb 11;8:67. doi: 10.3389/fchem.2020.00067. eCollection 2020.
Emission characteristics of heat recirculating porous burners with high temperature heat extraction are studied numerically. Two types of burners are considered: counterflow porous burner (CFB) and reciprocal counterflow porous burner (RCFB). The combustion of methane-air mixtures flowing through the porous media is modeled by solving steady state governing equations to obtain the flame temperature and species profiles. Formation of CO, NO, NO, and NO is studied in CFB and RCFB in a range of equivalence ratios from 0.3 to 1.0 and heat extraction temperatures from 300 to 1,300 K. The contribution of various NO formation mechanisms is comparatively analyzed and related to the NO generation predicted by a detailed chemistry mechanism. The effect of high temperature heat extraction on the formation of CO and NO is analyzed. Numerical predictions indicate a constant monotonic decrease of NO concentration with increasing temperature of energy extraction. The formation of CO is observed to follow the similar trend. For heat extraction at 1,300 K, simulations predicted 3.6 ppm of NO and 3.9 ppm of CO for CFB and 4.1 ppm of NO and 3.5 ppm of CO for RCFB when these burners are operated at an equivalence ratio of 0.7.
对具有高温热提取功能的热循环多孔燃烧器的排放特性进行了数值研究。考虑了两种类型的燃烧器:逆流多孔燃烧器(CFB)和往复逆流多孔燃烧器(RCFB)。通过求解稳态控制方程来模拟流经多孔介质的甲烷 - 空气混合物的燃烧,以获得火焰温度和物种分布。在当量比范围为0.3至1.0以及热提取温度为300至1300 K的条件下,研究了CFB和RCFB中CO、NO、NO和NO的形成。对各种NO形成机制的贡献进行了比较分析,并与详细化学机制预测的NO生成相关联。分析了高温热提取对CO和NO形成的影响。数值预测表明,随着能量提取温度的升高,NO浓度持续单调下降。观察到CO的形成遵循类似趋势。当这些燃烧器在当量比为0.7下运行时,对于1300 K的热提取,模拟预测CFB的NO为3.6 ppm,CO为3.9 ppm,RCFB的NO为4.1 ppm,CO为3.5 ppm。