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受人为因素影响的中国中部严重空气污染区:时空分布与潜在源。

A seriously air pollution area affected by anthropogenic in the central China: temporal-spatial distribution and potential sources.

机构信息

Key Laboratory for Yellow River and Huai River Water Environment and Pollution Control, Ministry of Education, Henan Key Laboratory for Environmental Pollution Control, School of Environment, Henan Normal University, Xinxiang, 453007, Henan, People's Republic of China.

College of Water Sciences, Beijing Normal University, Beijing, 100875, People's Republic of China.

出版信息

Environ Geochem Health. 2020 Oct;42(10):3199-3211. doi: 10.1007/s10653-020-00558-7. Epub 2020 Apr 18.

DOI:10.1007/s10653-020-00558-7
PMID:32306229
Abstract

This study used the officially released data by the Chinese air quality monitoring network to analyze the pollution characteristics of six air pollutants (PM, PM, SO, NO, CO, and O) for 29 cities in the Central Plains Economic Zone (CPEZ; China) in 2015. During 2015, serious particulate matter (PM) pollution often occurred, and the concentrations of PM and PM were 77 μg m and 128 μg m, respectively. Air pollutants were at higher concentrations in the northern cities than those in the southern region of the CPEZ, and the correlation among the cities indicated that there was regional pollution in CPEZ. Generally, PM, SO, NO, and CO showed similar seasonal characteristics and the highest and lowest concentrations appeared in winter and summer, respectively. In addition, we used the HYSPLIT model and trajStat model to identify the potential source contribution function and concentration-weighted trajectory of Zhengzhou, the central city of CPEZ. More serious air pollution occurred when air masses were transported from the west of the CPEZ. Shaanxi Province, Hubei Province, Anhui Province and the northwest of the CPEZ were found to be the main exogenous sources of total PM with contributions of > 100 μg m PM and > 180 μg m PM. Therefore, the concentrations of PM in 2015 at Zhengzhou were probably influenced by both long-distance transmission and local emissions.

摘要

本研究利用中国空气质量监测网络发布的官方数据,分析了 2015 年中原经济区(CPEZ;中国)29 个城市六种空气污染物(PM、PM、SO、NO、CO 和 O)的污染特征。2015 年期间,经常发生严重的颗粒物(PM)污染,PM 和 PM 的浓度分别为 77μg/m 和 128μg/m。北部城市的空气污染物浓度高于 CPEZ 南部地区,城市间的相关性表明 CPEZ 存在区域污染。一般来说,PM、SO、NO 和 CO 表现出相似的季节性特征,最高和最低浓度分别出现在冬季和夏季。此外,我们使用 HYSPLIT 模型和 trajStat 模型来识别中原经济区中心城市郑州的潜在源贡献函数和浓度加权轨迹。当空气团从 CPEZ 的西部输送时,会发生更严重的空气污染。陕西省、湖北省、安徽省和 CPEZ 的西北部被发现是总 PM 的主要外源,其贡献值分别大于 100μg/m PM 和大于 180μg/m PM。因此,2015 年郑州的 PM 浓度可能受到远距离传输和本地排放的共同影响。

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