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用于环境监测的β和γ辐照地质材料的热释光研究

Thermoluminescence Studies of β and γ-Irradiated Geological Materials for Environment Monitoring.

作者信息

Cheng-Lin Gu, Dubey Vikas, Kushwah Kamal Kumar, Mishra Manish Kumar, Pandey Ekta, Tiwari Ratnesh, Chandra Angesh, Dubey Neha

机构信息

Department of Environment, Faculty of Science, Jiamusi University, Jiamusi, 154007, China.

Department of Applied Physics; Bhilai Institute of Technology Raipur, Raipur, 493661, India.

出版信息

J Fluoresc. 2020 Jul;30(4):819-825. doi: 10.1007/s10895-020-02536-9. Epub 2020 May 20.

Abstract

In the present report, thermally stimulated luminescence (TSL) of quartz and limestone samples irradiated with β and γ-rays has been investigated. Herein the formation of trap depths and calculation of kinetic parameters of β and γ - irradiated quartz and limestone samples were studied through thermoluminescence (TL) glow curve analyses. The quartz and limestone samples were collected from various sites of Chhattisgarh (Patharia and Dalli-Rajhara mines). The collected raw samples were annealed at 400 °C. The phase formation of collected samples is confirmed by X-ray diffraction studies. The grain sizes of the samples are determined by using Debye-Scherrer formula. TL glow curves of the collected samples were recorded for various doses of β and γ-rays. Kinetic parameters such as order of kinetics frequency factor and trap depth were calculated by employing CGCD methods. A comparative study on the TL properties of the geological materials under β and γ-irradiation was done. The trap model analysis was executed to determine the nature of traps responsible for dominant TL peaks of β and γ-irradiated limestone and quartz samples.

摘要

在本报告中,对用β射线和γ射线辐照的石英和石灰石样品的热激发发光(TSL)进行了研究。在此,通过热释光(TL)发光曲线分析研究了β射线和γ射线辐照的石英和石灰石样品的陷阱深度形成以及动力学参数的计算。石英和石灰石样品采集自恰蒂斯加尔邦的不同地点(帕塔里亚和达利 - 拉杰哈拉矿)。采集的原始样品在400℃下退火。通过X射线衍射研究确认了采集样品的相形成。使用德拜 - 谢乐公式确定样品的晶粒尺寸。记录了采集样品在不同剂量β射线和γ射线下的TL发光曲线。采用CGCD方法计算了动力学级数、频率因子和陷阱深度等动力学参数。对β射线和γ射线辐照下地质材料的TL特性进行了比较研究。进行了陷阱模型分析,以确定导致β射线和γ射线辐照的石灰石和石英样品主要TL峰的陷阱性质。

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