Faculty of Chemistry, Adam Mickiewicz University, Uniwersytetu Poznańskiego 8, 61-614, Poznań, Poland.
Chair and Department of Genetics and Pharmaceutical Microbiology, Poznań University of Medical Sciences (PUMS), Święcickiego 4, 60-781, Poznań, Poland.
ChemMedChem. 2020 Aug 19;15(16):1529-1551. doi: 10.1002/cmdc.202000273. Epub 2020 Jun 12.
Desosamines of azithromycin (AZM) and clarithromycin (CLA) were modified by N-alkylation or nucleophilic substitution at the carbonyl/CuAAC sequence. Biological studies revealed a higher antibacterial potency of quaternary N-alkylammonium bromides of CLA as compared to AZM. SAR studies of CLA salts, including biological, conformation and molecular-docking analysis, enriched by physicochemical parameters, showed the importance of less bulky and unsaturated substituent for an efficient docking mode at the ribosomal tunnel and good antibacterial potency against clinical and standard Streptococcus pneumoniae and Streptococcus pyogenes strains (MICs 0.25 or 0.5 μg/mL). These CLA salts also have an at least threefold lower cytotoxicity than reference antibiotics at comparable antibacterial activity against the S. pneumoniae clinical strain. Differences in antibacterial effects noted for AZM and CLA salts bearing less bulky N-substituents can be better understood when their binding modes in the ribosomal tunnel are considered rather than their common low lipophilicity and excellent water solubility.
阿奇霉素(AZM)和克拉霉素(CLA)的去氧氨基糖经 N-烷基化或亲核取代羰基/CuAAC 序列修饰。生物研究表明,与 AZM 相比,CLA 的季铵盐具有更高的抗菌活性。CLA 盐的 SAR 研究,包括生物、构象和分子对接分析,以及物理化学参数的补充,表明对于在核糖体隧道中有效的对接模式和针对临床和标准肺炎链球菌和化脓性链球菌菌株的良好抗菌活性,较小和不饱和取代基的重要性(MICs 为 0.25 或 0.5μg/mL)。与具有可比抗菌活性的参考抗生素相比,这些 CLA 盐的细胞毒性至少低三倍,对肺炎链球菌临床株的抗菌作用。当考虑到它们在核糖体隧道中的结合模式而不是它们常见的低脂溶性和极好的水溶性时,可以更好地理解 AZM 和 CLA 盐的抗菌作用的差异,这些盐带有较小的 N-取代基。