Kang Hui Peng, Chen Shi, Chu Wei, Yao Jin Ping, Chen Jing, Liu Xiao Jun, Cheng Ya, Xu Zhi Zhan
Opt Express. 2020 Jun 22;28(13):19325-19333. doi: 10.1364/OE.397488.
A systematic study of nonsequential double ionization (NSDI) of alkaline-earth metal atoms with mid-infrared femtosecond pulses is reported. We find that the measured NSDI yield shows a strong target dependence and it is more suppressed for alkaline-earth metal with higher ionization potential. The observation is attributed to the differences in the recollision induced excitation and ionization cross sections of alkaline-earth metals. This work indicates that NSDI of alkaline-earth metals can be generally understood within recollision picture and sheds light on ultrafast control of electron correlation and dynamics of ionic excited states during NSDI of atoms with complex structures.
报道了一项关于用中红外飞秒脉冲对碱土金属原子进行非顺序双电离(NSDI)的系统研究。我们发现,测量得到的NSDI产率表现出强烈的靶依赖性,并且对于具有较高电离势的碱土金属,其产率受到的抑制更大。该观察结果归因于碱土金属在再碰撞诱导激发和电离截面方面的差异。这项工作表明,碱土金属的NSDI通常可以在再碰撞图像中得到理解,并为具有复杂结构的原子在NSDI过程中的电子关联超快控制以及离子激发态动力学提供了启示。