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非顺序双电离中轨道角动量的纠缠

Entanglement of orbital angular momentum in non-sequential double ionization.

作者信息

Maxwell Andrew S, Madsen Lars Bojer, Lewenstein Maciej

机构信息

ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, Av. Carl Friedrich Gauss 3, 08860, Castelldefels, Barcelona, Spain.

Department of Physics and Astronomy, Aarhus University, DK-8000, Aarhus C, Denmark.

出版信息

Nat Commun. 2022 Aug 10;13(1):4706. doi: 10.1038/s41467-022-32128-z.

DOI:10.1038/s41467-022-32128-z
PMID:35948552
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9365801/
Abstract

Entanglement has a capacity to enhance imaging procedures, but this remains unexplored for attosecond imaging. Here, we elucidate that possibility, addressing orbital angular momentum (OAM) entanglement in ultrafast processes. In the correlated process non-sequential double ionization (NSDI) we demonstrate robust photoelectron entanglement. In contrast to commonly considered continuous variables, the discrete OAM allows for a simpler interpretation, computation, and measurement of entanglement. The logarithmic negativity reveals that the entanglement is robust to incoherence and an entanglement witness minimizes the number of measurements to detect the entanglement, both quantities are related to OAM coherence terms. We quantify the entanglement for a range of targets and field parameters to find the most entangled photoelectron pairs. This methodology provides a general way to use OAM to quantify and measure entanglement, well-suited to attosecond processes, and can be exploited to enhance imaging capabilities through correlated measurements, or for generation of OAM-entangled electrons.

摘要

纠缠具有增强成像过程的能力,但这在阿秒成像中仍未得到探索。在此,我们阐明了这种可能性,探讨了超快过程中的轨道角动量(OAM)纠缠。在关联过程非顺序双电离(NSDI)中,我们展示了稳健的光电子纠缠。与通常考虑的连续变量不同,离散的OAM允许对纠缠进行更简单的解释、计算和测量。对数负性表明该纠缠对非相干性具有稳健性,并且一个纠缠见证者可将检测纠缠所需的测量次数减至最少,这两个量都与OAM相干项相关。我们对一系列目标和场参数的纠缠进行了量化,以找到纠缠度最高的光电子对。这种方法提供了一种利用OAM来量化和测量纠缠的通用方法,非常适合阿秒过程,并且可通过关联测量来增强成像能力,或用于生成OAM纠缠电子。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/63a8/9365801/2da29f71a94d/41467_2022_32128_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/63a8/9365801/edf1967b08ea/41467_2022_32128_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/63a8/9365801/fc5503940f73/41467_2022_32128_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/63a8/9365801/2da29f71a94d/41467_2022_32128_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/63a8/9365801/edf1967b08ea/41467_2022_32128_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/63a8/9365801/fc5503940f73/41467_2022_32128_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/63a8/9365801/2da29f71a94d/41467_2022_32128_Fig3_HTML.jpg

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本文引用的文献

1
Experimental Control of Quantum-Mechanical Entanglement in an Attosecond Pump-Probe Experiment.阿秒泵浦-探测实验中量子力学纠缠的实验控制
Phys Rev Lett. 2022 Jan 28;128(4):043201. doi: 10.1103/PhysRevLett.128.043201.
2
Conservation laws for electron vortices in strong-field ionisation.强场电离中电子涡旋的守恒定律。
Eur Phys J D At Mol Opt Phys. 2021;75(7):199. doi: 10.1140/epjd/s10053-021-00214-4. Epub 2021 Jul 9.
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Control of Attosecond Entanglement and Coherence.阿秒纠缠与相干的控制
Light Sci Appl. 2024 Feb 1;13(1):41. doi: 10.1038/s41377-024-01381-w.
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Ultrafast preparation and detection of entangled atoms.纠缠原子的超快制备与探测。
Sci Adv. 2023 Sep 8;9(36):eabq8227. doi: 10.1126/sciadv.abq8227.
Phys Rev Lett. 2021 Mar 19;126(11):113203. doi: 10.1103/PhysRevLett.126.113203.
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Experimental Demonstration of an Electrostatic Orbital Angular Momentum Sorter for Electron Beams.用于电子束的静电轨道角动量分选器的实验演示。
Phys Rev Lett. 2021 Mar 5;126(9):094802. doi: 10.1103/PhysRevLett.126.094802.
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Manipulating twisted electrons in strong-field ionization.在强场电离中操控扭曲电子。
Faraday Discuss. 2021 May 27;228(0):394-412. doi: 10.1039/d0fd00105h.
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Quantum electronic coherences by attosecond transient absorption spectroscopy: B-spline RCS-ADC study.阿秒瞬态吸收光谱法研究量子电子相干性:B样条RCS-ADC研究
Faraday Discuss. 2021 May 27;228(0):286-311. doi: 10.1039/d0fd00104j.
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Nonsequential double ionization of alkaline-earth metal atoms by intense mid-infrared femtosecond pulses.强中红外飞秒脉冲对碱土金属原子的非顺序双电离
Opt Express. 2020 Jun 22;28(13):19325-19333. doi: 10.1364/OE.397488.
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It is all about phases: ultrafast holographic photoelectron imaging.一切都与相位有关:超快全息光电子成像。
Rep Prog Phys. 2020 Mar;83(3):034401. doi: 10.1088/1361-6633/ab5c91. Epub 2019 Nov 28.
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Symphony on strong field approximation.强场近似下的交响乐。
Rep Prog Phys. 2019 Nov;82(11):116001. doi: 10.1088/1361-6633/ab2bb1. Epub 2019 Jun 21.
10
Effects of core space and excitation levels on ground-state correlation and photoionization dynamics of Be and Ne.铍和氖的基态关联和光电离动力学的核空间和激发态水平的影响。
J Chem Phys. 2019 Feb 28;150(8):084305. doi: 10.1063/1.5082940.