Jiang X C, Zhou Y W, Gao D L, Huang Y, Gao L
Opt Express. 2020 Jun 8;28(12):17384-17394. doi: 10.1364/OE.394605.
We theoretically study the optical bistability and tristability in plasmonic coated nanospheres containing the nonlinear plasmonic shell and the dielectric core with radial anisotropy. Based on self-consistent mean-field approximation, we establish the relationship between the local field in the shell and the applied incident field, taking into account the Lorentz local field. One or two optical bistabilities and even optical tristability can be observed. Especially, there are two critical geometric parameters between which two optical bistabilities exist. Physically, two optical bistablities result from the excitations of two surface plasmonic resonant modes in the inner and outer interfaces of coated nanospheres, which are well reflected from the spectral representation with two poles. Moreover, the involvement of the radial anisotropy is quite essential to realize the optical tristability. Further discussion on the field-induced tuning of the reflectance reveals the macroscopic properties of this nonlinear optical structure, which provides a potential candidate for designing multi-stable optical devices at the nanoscale.
我们从理论上研究了包含非线性等离子体壳层和具有径向各向异性的电介质核的等离子体包覆纳米球中的光学双稳性和三稳性。基于自洽平均场近似,我们考虑了洛伦兹局部场,建立了壳层中的局部场与外加入射场之间的关系。可以观察到一个或两个光学双稳性,甚至光学三稳性。特别地,存在两个临界几何参数,在这两个参数之间存在两个光学双稳性。从物理角度来看,两个光学双稳性是由包覆纳米球内外界面处的两个表面等离子体共振模式的激发引起的,这在具有两个极点的光谱表示中得到了很好的体现。此外,径向各向异性的参与对于实现光学三稳性至关重要。对场诱导的反射率调谐的进一步讨论揭示了这种非线性光学结构的宏观特性,这为在纳米尺度上设计多稳态光学器件提供了一个潜在的候选方案。