Department of Environmental Sciences, University of Virginia, Charlottesville, Virginia 22904, United States.
Department of Public Health, Emory University, Atlanta, Georgia 30322, United States.
Environ Sci Technol. 2020 Aug 18;54(16):9882-9895. doi: 10.1021/acs.est.0c01864. Epub 2020 Aug 5.
Houston, Texas is a major U.S. urban and industrial area where poor air quality is unevenly distributed and a disproportionate share is located in low-income, non-white, and Hispanic neighborhoods. We have traditionally lacked city-wide observations to fully describe these spatial heterogeneities in Houston and in cities globally, especially for reactive gases like nitrogen dioxide (NO). Here, we analyze novel high-spatial-resolution (250 m × 500 m) NO vertical columns measured by the NASA GCAS airborne spectrometer as part of the September-2013 NASA DISCOVER-AQ mission and discuss differences in population-weighted NO at the census-tract level. Based on the average of 35 repeated flight circuits, we find 37 ± 6% higher NO for non-whites and Hispanics living in low-income tracts (LIN) compared to whites living in high-income tracts (HIW) and report NO disparities separately by race ethnicity (11-32%) and poverty status (15-28%). We observe substantial time-of-day and day-to-day variability in LIN-HIW NO differences (and in other metrics) driven by the greater prevalence of NO (≡NO + NO) emission sources in low-income, non-white, and Hispanic neighborhoods. We evaluate measurements from the recently launched satellite sensor TROPOMI (3.5 km × 7 km at nadir), averaged to 0.01° × 0.01° using physics-based oversampling, and demonstrate that TROPOMI resolves similar relative, but not absolute, tract-level differences compared to GCAS. We utilize the high-resolution FIVE and NEI NO inventories, plus one year of TROPOMI weekday-weekend variability, to attribute tract-level NO disparities to industrial sources and heavy-duty diesel trucking. We show that GCAS and TROPOMI spatial patterns correspond to the surface patterns measured using aircraft profiling and surface monitors. We discuss opportunities for satellite remote sensing to inform decision making in cities generally.
德克萨斯州休斯顿是美国一个主要的城市和工业地区,那里的空气质量分布不均,不成比例的部分位于低收入、非白人和西班牙裔社区。我们传统上缺乏全市范围的观测来充分描述休斯顿和全球城市的这些空间异质性,特别是对于氮氧化物(NO)等反应性气体。在这里,我们分析了 NASA GCAS 机载光谱仪在 2013 年 9 月 NASA DISCOVER-AQ 任务中测量的新型高空间分辨率(250 m×500 m)NO 垂直柱,并讨论了按人口加权的 NO 在普查区水平上的差异。基于 35 次重复飞行循环的平均值,我们发现,与居住在高收入区(HIW)的白人相比,居住在低收入区(LIN)的非白人和西班牙裔的 NO 水平高出 37±6%,并分别按种族(11-32%)和贫困状况(15-28%)报告 NO 差异。我们观察到,在低收入、非白人和西班牙裔社区中,NO 排放源更为普遍,导致 LIN-HIW 的 NO 差异(和其他指标)存在显著的昼夜和每日变化。我们评估了最近发射的卫星传感器 TROPOMI(在天底处为 3.5 km×7 km)的测量值,使用基于物理的过采样方法将其平均到 0.01°×0.01°,并证明 TROPOMI 与 GCAS 相比可以分辨出类似的相对但不是绝对的普查区差异。我们利用高分辨率 FIVE 和 NEI 的 NO 清单,以及一年的 TROPOMI 工作日-周末变化,将普查区的 NO 差异归因于工业源和重型柴油卡车。我们表明,GCAS 和 TROPOMI 的空间模式与使用飞机剖面和地面监测器测量的表面模式相对应。我们讨论了卫星遥感为城市决策提供信息的机会。