• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利:CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验

基于多组分多步动力学模型的生物质空气-蒸汽气化:一种生产富氢合成气的清洁策略。

Air-steam gasification of biomass based on a multi-composition multi-step kinetic model: A clean strategy for hydrogen-enriched syngas production.

机构信息

School of Mechatronic Engineering, Xian Technological University, Xian 710021, China.

School of Mechatronic Engineering, Xian Technological University, Xian 710021, China.

出版信息

Sci Total Environ. 2021 Jan 20;753:141690. doi: 10.1016/j.scitotenv.2020.141690. Epub 2020 Aug 13.

DOI:10.1016/j.scitotenv.2020.141690
PMID:32896730
Abstract

Biomass, as a renewable energy source, has high potential for supplying the energy needs of modern societies. Gasification is a thermochemical route for converting biomass into combustible gas at high temperatures. The main purpose of the present study was to develop an Aspen Plus model of air-steam gasification of biomass (sawdust) to predict the gasification characteristics and performances. The prediction capability of the model was evaluated by comparison with experimental data obtained in a fluidized bed biomass gasifier. First, the influence of gasification temperature on gas composition, product yields and gasifier performances was investigated. The biomass feeding rate and air flow rate were set at~0.445 kg/h and 0.5 Nm/h, respectively, while the gasifier temperature was varied between 700 °C to 800 °C. With the increase of temperature, the gas yield (DGY) increased steadily from 1.72 to 2.0 Nm/kg, while the HHV of the produced syngas (HHV) increased initially from 5.38 to 5.73 MJ/Nm and then decreased to 5.69 MJ/Nm. After determining optimal temperature (800 °C), the influence of equivalence ratio (ER) and steam/biomass ratio (S/B) on gasification characteristics, dry gas yield (DGY) and tar yield (TRY) was studied. As ER increased from 0.19 to 0.23, TRY decreased from 9.13 g/Nm to 8.45 g/Nm. In contrast, DGY initially increased from 2.02 Nm/kg to 2.43 Nm/kg as ER increased from 0.19 to 0.21 and then dropped to 2.24 Nm/kg at ER of 0.23. An increase in S/B from 0.61 to 2.7 also resulted in a slight increase in HHV; however, TRY showed a decreasing trend (from 9.65 g/Nm to 8.95 g/Nm). The results showed that the model developed in this paper is a promising tool for simulating the biomass gasification at various operating conditions.

摘要

生物质作为一种可再生能源,具有为现代社会提供能源需求的巨大潜力。气化是一种在高温下将生物质转化为可燃气体的热化学途径。本研究的主要目的是开发一种基于 Aspen Plus 的生物质(木屑)空气-蒸汽气化模型,以预测气化特性和性能。通过与流化床生物质气化炉获得的实验数据进行比较来评估模型的预测能力。首先,研究了气化温度对气体成分、产品收率和气化炉性能的影响。生物质进料速率和空气流量分别设定为~0.445kg/h 和 0.5Nm/h,而气化炉温度在 700°C 至 800°C 之间变化。随着温度的升高,气体产率(DGY)从 1.72 稳定增加到 2.0Nm/kg,而产生的合成气的高热值(HHV)最初从 5.38 增加到 5.73MJ/Nm,然后降低到 5.69MJ/Nm。在确定最佳温度(800°C)后,研究了当量比(ER)和蒸汽/生物质比(S/B)对气化特性、干气产率(DGY)和焦油产率(TRY)的影响。随着 ER 从 0.19 增加到 0.23,TRY 从 9.13g/Nm 降低到 8.45g/Nm。相反,随着 ER 从 0.19 增加到 0.21,DGY 从 2.02Nm/kg 增加到 2.43Nm/kg,然后在 ER 为 0.23 时降至 2.24Nm/kg。S/B 从 0.61 增加到 2.7 也导致 HHV 略有增加;然而,TRY 呈下降趋势(从 9.65g/Nm 降至 8.95g/Nm)。结果表明,本文开发的模型是在各种操作条件下模拟生物质气化的有前途的工具。

相似文献

1
Air-steam gasification of biomass based on a multi-composition multi-step kinetic model: A clean strategy for hydrogen-enriched syngas production.基于多组分多步动力学模型的生物质空气-蒸汽气化:一种生产富氢合成气的清洁策略。
Sci Total Environ. 2021 Jan 20;753:141690. doi: 10.1016/j.scitotenv.2020.141690. Epub 2020 Aug 13.
2
Characteristics of hydrogen energy yield in steam gasification of coffee residues.咖啡渣蒸汽气化制氢产率的特性
Environ Sci Pollut Res Int. 2024 May;31(23):33807-33818. doi: 10.1007/s11356-024-33499-0. Epub 2024 Apr 30.
3
Steam-air fluidized bed gasification of distillers grains: Effects of steam to biomass ratio, equivalence ratio and gasification temperature.酒糟的蒸汽-空气流化床气化:蒸汽与生物质比、当量比及气化温度的影响
Bioresour Technol. 2009 Mar;100(6):2062-8. doi: 10.1016/j.biortech.2008.10.011. Epub 2008 Nov 22.
4
Torrefaction/carbonization-enhanced gasification-steam reforming of biomass for promoting hydrogen-enriched syngas production and tar elimination over gasification biochars.生物质的热解/碳化增强气化-蒸汽重整促进富氢合成气生产和气化生物炭中焦油消除。
Bioresour Technol. 2022 Nov;363:127960. doi: 10.1016/j.biortech.2022.127960. Epub 2022 Sep 13.
5
Steam gasification of acid-hydrolysis biomass CAHR for clean syngas production.酸解生物质 CAHR 的蒸汽气化用于清洁合成气生产。
Bioresour Technol. 2015 Mar;179:323-330. doi: 10.1016/j.biortech.2014.12.039. Epub 2014 Dec 18.
6
Hydrogen-rich gas production by steam gasification of char from biomass fast pyrolysis in a fixed-bed reactor: influence of temperature and steam on hydrogen yield and syngas composition.在固定床反应器中通过生物质快速热解的炭进行水蒸气气化制富氢气体:温度和水蒸气对产氢量和合成气组成的影响。
Bioresour Technol. 2010 Jul;101(14):5633-7. doi: 10.1016/j.biortech.2010.02.025. Epub 2010 Mar 2.
7
An experimental study on biomass air-steam gasification in a fluidized bed.流化床中生物质空气-蒸汽气化的实验研究
Bioresour Technol. 2004 Oct;95(1):95-101. doi: 10.1016/j.biortech.2004.02.003.
8
Characterization of a dual fluidized bed gasifier with blended biomass/coal as feedstock.以生物质/煤混合原料为燃料的双流化床气化炉的特性研究。
Bioresour Technol. 2018 Apr;254:97-106. doi: 10.1016/j.biortech.2018.01.067. Epub 2018 Feb 2.
9
Investigation on biomass steam gasification in a dual fluidized bed reactor with the granular kinetic theory.采用颗粒动理学理论对双流化床中生物质蒸汽气化进行研究。
Bioresour Technol. 2018 Dec;269:384-392. doi: 10.1016/j.biortech.2018.08.099. Epub 2018 Aug 31.
10
Experimental and predicted approaches for biomass gasification with enriched air-steam in a fluidised bed.流化床中富氧空气-蒸汽生物质气化的实验与预测方法
Waste Manag Res. 2014 Oct;32(10):988-96. doi: 10.1177/0734242X14552555. Epub 2014 Sep 29.

引用本文的文献

1
Chemical Kinetic Modeling of Air-Steam Gasification of Eucalyptus Wood Sawdust for H-Rich Syngas Production.用于生产富氢合成气的桉木锯末空气-蒸汽气化的化学动力学建模
ACS Omega. 2023 Mar 31;8(14):13396-13409. doi: 10.1021/acsomega.3c00908. eCollection 2023 Apr 11.
2
H-rich syngas production from gasification involving kinetic modeling: RSM-utility optimization and techno-economic analysis.基于动力学模型的气化制富氢合成气:响应曲面法-效用优化及技术经济分析
RSC Adv. 2023 Mar 31;13(15):10308-10321. doi: 10.1039/d3ra00287j. eCollection 2023 Mar 27.