Eco-Friendly New Materials Research Center, Therapeutics&Biotechnology Division, Korea Research Institute of Chemical Technology(KRICT), 141 Gajeong-ro, Yuseong-gu, Daejeon 34114, Republic of Korea.
Department of Chemistry, Korea University, 145 Anam-ro, Seongbuk-gu, Seoul 02841, Republic of Korea.
Org Lett. 2020 Oct 2;22(19):7465-7469. doi: 10.1021/acs.orglett.0c02603. Epub 2020 Sep 15.
A new protocol for preparation of acyl fluorides was developed by recognizing activated ketones as starting materials. The method provides a different scope compared with previously reported methods that employ carboxylic acids as substrates. A working hypothesis of pull-and-push-driven fluorinative C-C bond cleavage was successfully demonstrated by the simple addition of diethylaminosulfur trifluoride (DAST) derivatives to α-oximinoketones. The designed reaction system led to a highly efficient and chemoselective reaction. The wide availability of the ketones allowed for a range of synthetically useful aryloyl and aliphatic acyl fluorides including those containing chiral skeletons. The method is mild, fast, scalable, and potentially one-pot operative.
我们开发了一种新的酰氟制备方法,该方法以活化酮作为起始原料。与之前使用羧酸作为底物的报道方法相比,该方法提供了不同的应用范围。通过将二乙氨基三氟化硫(DAST)衍生物简单地添加到α-氧亚氨基酮中,成功地证明了推拉驱动的氟化 C-C 键断裂的工作假说。设计的反应体系导致高效和选择性的反应。酮的广泛可得性允许合成一系列有用的芳基和脂肪酰氟化物,包括含有手性骨架的酰氟化物。该方法温和、快速、可扩展,并且具有潜在的一锅操作能力。