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本文引用的文献

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Asteroid impact, not volcanism, caused the end-Cretaceous dinosaur extinction.小行星撞击而非火山活动导致了白垩纪末期恐龙灭绝。
Proc Natl Acad Sci U S A. 2020 Jul 21;117(29):17084-17093. doi: 10.1073/pnas.2006087117. Epub 2020 Jun 29.
2
A steeply-inclined trajectory for the Chicxulub impact.一个陡峭倾斜的 Chicxulub 撞击轨迹。
Nat Commun. 2020 May 26;11(1):1480. doi: 10.1038/s41467-020-15269-x.
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The first day of the Cenozoic.新生代的第一天。
Proc Natl Acad Sci U S A. 2019 Sep 24;116(39):19342-19351. doi: 10.1073/pnas.1909479116. Epub 2019 Sep 9.
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Black carbon lofts wildfire smoke high into the stratosphere to form a persistent plume.黑碳排放物将野火烟雾高高地送入平流层,形成持久的羽流。
Science. 2019 Aug 9;365(6453):587-590. doi: 10.1126/science.aax1748.
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Source identification of polycyclic aromatic hydrocarbons in soil sediments: Application of different methods.土壤沉积物中多环芳烃的来源识别:不同方法的应用。
Sci Total Environ. 2019 Feb 20;652:1077-1089. doi: 10.1016/j.scitotenv.2018.10.014. Epub 2018 Oct 12.
6
Rapid recovery of life at ground zero of the end-Cretaceous mass extinction.白垩纪末大灭绝“震中”地带生命的快速恢复。
Nature. 2018 Jun;558(7709):288-291. doi: 10.1038/s41586-018-0163-6. Epub 2018 May 30.
7
On transient climate change at the Cretaceous-Paleogene boundary due to atmospheric soot injections.因大气烟尘注入而导致白垩纪-古近纪界线时期的气候瞬间变化
Proc Natl Acad Sci U S A. 2017 Sep 5;114(36):E7415-E7424. doi: 10.1073/pnas.1708980114. Epub 2017 Aug 21.
8
The formation of peak rings in large impact craters.大型撞击坑中环峰的形成。
Science. 2016 Nov 18;354(6314):878-882. doi: 10.1126/science.aah6561.
9
Global climate change driven by soot at the K-Pg boundary as the cause of the mass extinction.白垩纪-古近纪界线处烟灰导致的全球气候变化是物种大灭绝的原因。
Sci Rep. 2016 Jul 14;6:28427. doi: 10.1038/srep28427.
10
Chemical composition of floating and sunken in-situ burn residues from the Deepwater Horizon oil spill.墨西哥湾深海地平线溢油事件浮油和沉油原位燃烧残余物的化学成分分析。
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希克苏鲁伯陨石坑的有机物加剧了 K-Pg 撞击冬季。

Organic matter from the Chicxulub crater exacerbated the K-Pg impact winter.

机构信息

Department of Geosciences, The Pennsylvania State University, University Park, PA 16802;

Department of Geosciences, The Pennsylvania State University, University Park, PA 16802.

出版信息

Proc Natl Acad Sci U S A. 2020 Oct 13;117(41):25327-25334. doi: 10.1073/pnas.2004596117. Epub 2020 Sep 28.

DOI:10.1073/pnas.2004596117
PMID:32989138
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7568312/
Abstract

An asteroid impact in the Yucatán Peninsula set off a sequence of events that led to the Cretaceous-Paleogene (K-Pg) mass extinction of 76% species, including the nonavian dinosaurs. The impact hit a carbonate platform and released sulfate aerosols and dust into Earth's upper atmosphere, which cooled and darkened the planet-a scenario known as an impact winter. Organic burn markers are observed in K-Pg boundary records globally, but their source is debated. If some were derived from sedimentary carbon, and not solely wildfires, it implies soot from the target rock also contributed to the impact winter. Characteristics of polycyclic aromatic hydrocarbons (PAHs) in the Chicxulub crater sediments and at two deep ocean sites indicate a fossil carbon source that experienced rapid heating, consistent with organic matter ejected during the formation of the crater. Furthermore, PAH size distributions proximal and distal to the crater indicate the ejected carbon was dispersed globally by atmospheric processes. Molecular and charcoal evidence indicates wildfires were also present but more delayed and protracted and likely played a less acute role in biotic extinctions than previously suggested. Based on stratigraphy near the crater, between 7.5 × 10 and 2.5 × 10 g of black carbon was released from the target and ejected into the atmosphere, where it circulated the globe within a few hours. This carbon, together with sulfate aerosols and dust, initiated an impact winter and global darkening that curtailed photosynthesis and is widely considered to have caused the K-Pg mass extinction.

摘要

在尤卡坦半岛的一次小行星撞击引发了一系列事件,导致了白垩纪-古近纪(K-Pg)大规模物种灭绝,包括非鸟类恐龙。这次撞击袭击了一个碳酸盐台地,将硫酸盐气溶胶和尘埃释放到地球的高层大气中,导致地球冷却和变暗——这种情况被称为撞击冬季。全球范围内的 K-Pg 边界记录中都观察到了有机燃烧标记物,但它们的来源存在争议。如果其中一些是由沉积碳而不是野火产生的,那么这意味着来自靶岩的煤烟也促成了撞击冬季。奇克苏鲁布陨石坑沉积物和两个深海地点的多环芳烃(PAHs)特征表明,存在经历了快速加热的化石碳源,与在陨石坑形成过程中喷出的有机物一致。此外,陨石坑附近和远处的 PAH 粒径分布表明,喷出的碳通过大气过程在全球范围内分散。分子和木炭证据表明,野火也存在,但更迟且持续时间更长,而且在生物灭绝中的作用可能不如先前认为的那么急性。根据陨石坑附近的地层,从靶体中释放并喷射到大气中的黑碳有 7.5×10 和 2.5×10 g,在几小时内就在全球范围内循环。这种碳与硫酸盐气溶胶和尘埃一起引发了撞击冬季和全球变暗,从而减少了光合作用,这被广泛认为是导致 K-Pg 大规模灭绝的原因。