Zeng Yuqi, Pan Weijian, Ding Na, Kang Yuan, Man Yu Bon, Zeng Lixuan, Zhang Qiuyun, Luo Jiwen
School of Environment, South China Normal University, Higher Education Mega Center, Guangzhou, PR China.
Guangdong Engineering Technology Research Center for Drinking Water Safety, School of Environment, South China Normal University, Higher Education Mega Center, Guangzhou, PR China.
J Environ Sci Health A Tox Hazard Subst Environ Eng. 2020;55(13):1528-1533. doi: 10.1080/10934529.2020.1826191. Epub 2020 Sep 29.
Brominated flame retardants (BFRs) in house dust have raised significant concern around the world. However, few studies have reported the correlation between BFR concentrations in house dust and children's hair samples. In this study, BFR concentrations in house dust and children's hair were measured. Chemical analysis showed that the total concentrations of polybrominated diphenyl ethers (PBDEs) in house dust ranged from 334 to 4444 ng g, with a median of 442 ng g, and the concentrations in children's hair ranged from 352 to 655 ng g, with a median of 530 ng g. In addition, two alternative flame retardants, pentabromoethylbenzene (PBEB) and hexabromobenzene, were frequently detected in house dust and human hair. BDE209 was the most abundant PBDE congener detected in both house dust and children's hair. A significant correlation was found between the integrated PCA score of BFR concentrations in house dust and in children's hair ( = 0.31, < 0.05), indicating the great contribution of house dust to the bodily burden of PBDEs in children. Risk assessment indicated that children's exposure to PBDEs via non-dietary intake of house dust should be recognized as an important exposure pathway.
室内灰尘中的溴化阻燃剂(BFRs)已引起全球广泛关注。然而,很少有研究报道室内灰尘中BFR浓度与儿童头发样本之间的相关性。在本研究中,对室内灰尘和儿童头发中的BFR浓度进行了测量。化学分析表明,室内灰尘中多溴二苯醚(PBDEs)的总浓度范围为334至4444 ng/g,中位数为442 ng/g,儿童头发中的浓度范围为352至655 ng/g,中位数为530 ng/g。此外,两种替代阻燃剂,五溴乙苯(PBEB)和六溴苯,在室内灰尘和人发中经常被检测到。BDE209是在室内灰尘和儿童头发中检测到的最丰富的PBDE同系物。室内灰尘和儿童头发中BFR浓度的综合主成分分析(PCA)得分之间存在显著相关性(r = 0.31,p < 0.05),表明室内灰尘对儿童体内PBDEs负担有很大贡献。风险评估表明,应将儿童通过非饮食摄入室内灰尘接触PBDEs视为重要的暴露途径。