Shen Tien-Lin, Hu Han-Wen, Lin Wei-Ju, Liao Yu-Ming, Chen Tzu-Pei, Liao Yu-Kuang, Lin Tai-Yuan, Chen Yang-Fang
Graduate Institute of Applied Physics, National Taiwan University, Taipei 10617, Taiwan.
Department of Physics, National Taiwan University, Taipei 10617, Taiwan.
Sci Adv. 2020 Oct 7;6(41). doi: 10.1126/sciadv.aba1705. Print 2020 Oct.
The many distinct advantages of random lasers focused efforts on developing a breakthrough from optical pumping to electrical pumping. However, progress in these is limited due to high optical loss and low gain. In this work, we demonstrate an electrically pumped quantum dot (QD) random laser with visible emission based on a previously unexplored paradigm named coherent Förster resonance energy transfer (CFRET). In the CFRET process, when a coherent photonic mode is formed because of multiple scattering of the emitted light traveling in mixed donor and acceptor QDs, the donor QDs not only serve as scattering centers but are also enable coherent energy transfer to acceptor QDs. Therefore, the laser action can be easily achieved, and the lasing threshold is greatly reduced. Our approach of electrically pumped QD-based random lasers represents a substantial step toward a full-spectrum random laser for practical applications.
随机激光器的诸多显著优势促使人们致力于从光泵浦到电泵浦的突破。然而,由于高光学损耗和低增益,这些方面的进展有限。在这项工作中,我们基于一种名为相干福斯特共振能量转移(CFRET)的此前未被探索的范式,展示了一种具有可见发射的电泵浦量子点(QD)随机激光器。在CFRET过程中,当由于在混合供体和受体量子点中传播的发射光的多次散射而形成相干光子模式时,供体量子点不仅作为散射中心,还能实现向受体量子点的相干能量转移。因此,可以轻松实现激光作用,并且大大降低了激光阈值。我们基于电泵浦量子点的随机激光器方法代表了朝着用于实际应用的全光谱随机激光器迈出的重要一步。