Cascaded nonlinearity induced spatial domain effects in a high power femtosecond optical parametric oscillator.

We have investigated the effect of cascaded optical nonlinearity on the spatial beam properties of a femtosecond optical parametric oscillator (OPO). The OPO was operated with a tunable phase mismatch by varying the angle of the nonlinear crystal. The cascaded nonlinearity induced self-focusing and defocusing changed resonator's stability and impacted mode properties. With tuning of a phase mismatch, the calculated parabolic part of cascaded nonlinearity lens focal length changes from f ∼ 30 mm (D ∼ 33 m at Δθ ∼ -0.5) to infinity and back to f ∼ -110 mm (D ∼ -9 m at Δθ ∼ 0.9) in the LBO nonlinear crystal. Such high power nonlinear lenses in a cavity operated near its stability limit promoted the generation of axially asymmetric or pass-to-pass unstable resonator modes. It was shown that phase mismatched optical parametric oscillation changes the physical character of the resonator from linear to ring-like with two nonlinear crystals having two different focusing powers. Calculations showed that the QCN induced spatial nonlinear phase should lead to severe longitudinal chromatic aberrations for broad spectrum pulses. A numerical simulation in XYZ spatial domain and calculations using ABCD matrix approach confirmed the physical mechanisms underlying the experimental results and allowed for the interpretation of the observed effects.