Gunnink Pieter M, Bouwmeester Rosa Luca, Brinkman Alexander
Faculty of Science and Technology and MESA+ Institute for Nanotechnology, University of Twente, 7500 AE Enschede, The Netherlands.
J Phys Condens Matter. 2020 Feb 24;33(8):085601. doi: 10.1088/1361-648X/abc973.
In the quest for topological insulators with large band gaps, heterostructures with Rashba spin-orbit interactions come into play. Transition metal oxides with heavy ions are especially interesting in this respect. We discuss the design principles for stacking oxide Rashba layers. Assuming a single layer with a two-dimensional electron gas (2DEG) on both interfaces as a building block, a two-dimensional topological insulating phase is present when negative coupling between the 2DEGs exists. When stacking multiple building blocks, a two-dimensional or three-dimensional topological insulator is artificially created, depending on the intra- and interlayer coupling strengths and the number of building blocks. We show that the three-dimensional topological insulator is protected by reflection symmetry, and can therefore be classified as a topological crystalline insulator. In order to isolate the topological states from bulk states, the intralayer coupling term needs to be quadratic in momentum. It is described how such a quadratic coupling could potentially be realized by taking buckling within the layers into account. The buckling, thereby, brings the idea of stacked Rashba system very close to the alternative approach of realizing the buckled honeycomb lattice in [111]-oriented perovskite oxides.
在寻找具有大带隙的拓扑绝缘体的过程中,具有Rashba自旋轨道相互作用的异质结构发挥了作用。在这方面,含有重离子的过渡金属氧化物尤其引人关注。我们讨论了堆叠氧化物Rashba层的设计原则。假设以在两个界面上都具有二维电子气(2DEG)的单层作为构建单元,当2DEG之间存在负耦合时,就会出现二维拓扑绝缘相。当堆叠多个构建单元时,根据层内和层间耦合强度以及构建单元的数量,可以人为地创建二维或三维拓扑绝缘体。我们表明,三维拓扑绝缘体受反射对称性保护,因此可归类为拓扑晶体绝缘体。为了将拓扑态与体态隔离开来,层内耦合项在动量上需要是二次的。文中描述了如何通过考虑层内的屈曲来潜在地实现这种二次耦合。因此,屈曲使堆叠Rashba系统的概念与在[111]取向的钙钛矿氧化物中实现屈曲蜂窝晶格的另一种方法非常接近。