Hubei Key Laboratory of Mineral Resources Processing and Environment, Wuhan University of Technology, 122 Luoshi Road, Wuhan, Hubei, 430070, China; School of Resources and Environmental Engineering, Wuhan University of Technology, 122 Luoshi Road, Wuhan, Hubei, 430070, China.
Hubei Key Laboratory of Mineral Resources Processing and Environment, Wuhan University of Technology, 122 Luoshi Road, Wuhan, Hubei, 430070, China; School of Resources and Environmental Engineering, Wuhan University of Technology, 122 Luoshi Road, Wuhan, Hubei, 430070, China.
Chemosphere. 2021 Mar;267:128900. doi: 10.1016/j.chemosphere.2020.128900. Epub 2020 Nov 13.
Solid wastes are generated from human activities which could cause damage to the ecological environment and human beings. In recent years, there has been extensive research on solid wastes utilized as precursors, aggregates, fibers, etc. to prepare the geopolymers, which has invariably been a research hotspot. This review classifies the solid wastes utilized for geopolymers into three main categories: industrial waste, agricultural waste, and municipal waste. Accordingly, we systematically dissert solid wastes-based geopolymer from the perspectives of structure, properties, and application. The chemical composition, morphology, particle size, thermal conductivity, and other characteristics of solid wastes can trigger changes in the specific properties of geopolymers. On this account, solid wastes-based geopolymers have great potential in the domain of concrete, fireproof materials, impermeable materials, catalysts, adsorbents, and energy storage materials, etc. More importantly, geopolymers have obvious advantages in immobilizing heavy metals in solid wastes. Therefore, it can demonstrate geopolymer is a sustainable and environmentally friendly "green material". However, it still confronts the challenges of solid wastes utilized in geopolymer (technology, economy, administration). It requires the government, enterprises, and the public to work together for co-governance to accomplish industrialization and commercialization of solid wastes-based geopolymer.
固体废物是人类活动产生的,可能会对生态环境和人类造成损害。近年来,人们广泛研究了将固体废物用作前体、骨料、纤维等制备地聚合物,这一直是一个研究热点。本文将用于地聚合物的固体废物分为工业废物、农业废物和城市废物三类。相应地,我们从结构、性能和应用等方面对地聚物进行了系统的论述。固体废物的化学组成、形态、粒径、导热系数等特性会引发地聚合物特定性能的变化。因此,基于固体废物的地聚合物在混凝土、防火材料、不透水材料、催化剂、吸附剂和储能材料等领域具有巨大的潜力。更重要的是,地聚合物在地聚物中固化重金属方面具有明显的优势。因此,可以证明地聚合物是一种可持续的环保“绿色材料”。然而,它仍然面临着地聚合物中利用固体废物的挑战(技术、经济、管理)。这需要政府、企业和公众共同合作,实现基于固体废物的地聚合物的产业化和商业化。