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具有长程幂律相关弹性无序的非晶态固体的振动态密度。

Vibrational density of states of amorphous solids with long-ranged power-law-correlated disorder in elasticity.

作者信息

Cui Bingyu, Zaccone Alessio

机构信息

Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, CB3 0HE, Cambridge, UK.

Department of Physics "A. Pontremoli", University of Milan, via Celoria 16, 20133, Milano, Italy.

出版信息

Eur Phys J E Soft Matter. 2020 Nov 23;43(11):72. doi: 10.1140/epje/i2020-11995-2.

Abstract

A theory of vibrational excitations based on power-law spatial correlations in the elastic constants (or equivalently in the internal stress) is derived, in order to determine the vibrational density of states D([Formula: see text]) of disordered solids. The results provide the first prediction of a boson peak in amorphous materials where spatial correlations in the internal stresses (or elastic constants) are of power-law form, as is often the case in experimental systems, leading to a logarithmic enhancement of (Rayleigh) phonon attenuation. A logarithmic correction of the form [Formula: see text] is predicted to occur in the plot of the reduced excess DOS for frequencies around the boson peak in 3D. Moreover, the theory provides scaling laws of the density of states in the low-frequency region, including a [Formula: see text] regime in 3D, and provides information about how the boson peak intensity depends on the strength of power-law decay of fluctuations in elastic constants or internal stress. Analytical expressions are also derived for the dynamic structure factor for longitudinal excitations, which include a logarithmic correction factor, and numerical calculations are presented supporting the assumptions used in the theory.

摘要

为了确定无序固体的振动态密度(D(\omega)),我们推导了一种基于弹性常数(或等效地基于内应力)的幂律空间相关性的振动激发理论。结果首次预测了非晶材料中的玻色子峰,其中内应力(或弹性常数)的空间相关性呈幂律形式,这在实验系统中经常出现,导致(瑞利)声子衰减呈对数增强。预计在三维中玻色子峰附近频率的约化过剩态密度图中会出现形式为(\log(\omega / \omega_0))的对数修正。此外,该理论提供了低频区域态密度的标度律,包括三维中的(\omega^2) regime,并提供了有关玻色子峰强度如何依赖于弹性常数或内应力波动的幂律衰减强度的信息。还推导了纵向激发的动态结构因子的解析表达式,其中包括一个对数修正因子,并给出了数值计算结果以支持该理论中使用的假设。

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