Streubel Robert, Bouma D Simca, Bruni Frank, Chen Xiaoqian, Ercius Peter, Ciston Jim, N'Diaye Alpha T, Roy Sujoy, Kevan Steve D, Fischer Peter, Hellman Frances
Department of Physics and Astronomy, and Nebraska, Center for Materials and Nanoscience, University of Nebraska-Lincoln, Lincoln, NE, 68588, USA.
Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.
Adv Mater. 2021 Feb;33(8):e2004830. doi: 10.1002/adma.202004830. Epub 2021 Jan 12.
Topological solitary fields, such as magnetic and polar skyrmions, are envisioned to revolutionize microelectronics. These configurations have been stabilized in solid-state materials with a global inversion symmetry breaking, which translates in magnetic materials into a vector spin exchange known as the Dzyaloshinskii-Moriya interaction (DMI), as well as spin chirality selection and isotropic solitons. This work reports experimental evidence of 3D chiral spin textures, such as helical spins and skyrmions with different chirality and topological charge, stabilized in amorphous Fe-Ge thick films. These results demonstrate that structurally and chemically disordered materials with a random DMI can resemble inversion symmetry broken systems with similar magnetic properties, moments, and states. Disordered systems are distinguished from systems with global inversion symmetry breaking by their degenerate spin chirality that allows for forming isotropic and anisotropic topological spin textures at remanence, while offering greater flexibility in materials synthesis, voltage, and strain manipulation.
诸如磁斯格明子和极斯格明子等拓扑孤立场被认为将给微电子学带来变革。这些构型已在具有全局反演对称性破缺的固态材料中得以稳定,这在磁性材料中表现为一种称为Dzyaloshinskii-Moriya相互作用(DMI)的矢量自旋交换,以及自旋手性选择和各向同性孤子。这项工作报道了在非晶态Fe-Ge厚膜中稳定存在的三维手性自旋纹理的实验证据,例如具有不同手性和拓扑电荷的螺旋自旋和斯格明子。这些结果表明,具有随机DMI的结构和化学无序材料可以类似于具有相似磁性、磁矩和磁态的反演对称性破缺系统。无序系统与具有全局反演对称性破缺的系统的区别在于其简并自旋手性,这使得在剩余状态下能够形成各向同性和各向异性拓扑自旋纹理,同时在材料合成、电压和应变操控方面提供了更大的灵活性。