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具有双交联网络的超柔韧、耐疲劳、自修复 PVA/木聚糖/硼砂水凝胶。

Super flexible, fatigue resistant, self-healing PVA/xylan/borax hydrogel with dual-crosslinked network.

机构信息

College of Light Industry and Food Engineering, Guangxi University, Nanning 530004, PR China.

College of Light Industry and Food Engineering, Guangxi University, Nanning 530004, PR China.

出版信息

Int J Biol Macromol. 2021 Mar 1;172:66-73. doi: 10.1016/j.ijbiomac.2021.01.038. Epub 2021 Jan 9.

DOI:10.1016/j.ijbiomac.2021.01.038
PMID:33434549
Abstract

The high mechanical strength and self-healing properties of hydrogels are the focus of tissue engineering and biomedical research. Furthermore, the incompatibility between hydrogel toughness and self-healing has not been resolved. It is noteworthy that the double network (DN) hydrogels show great promise as a viable method for producing self-healing hydrogels with the above properties. The Xylan/PVA/Borax DN hydrogel was prepared by the one-pot method, shows various excellent performances, including strong strength (ca. 81 kPa), high toughness (ca.1652.42 kJ/m), good self-recovery (ca. 79% recovery), and excellent self-healing properties (self-healing efficiency reached to 85.8% for 30 s). This study proposes a strategy to design high strength, high toughness, large extensibility, and self-healing properties hydrogels based on xylan.

摘要

水凝胶的高强度和自修复性能是组织工程和生物医学研究的重点。此外,水凝胶韧性和自修复之间的不兼容尚未得到解决。值得注意的是,双网络(DN)水凝胶作为一种可行的方法,有望制备具有上述性能的自修复水凝胶。通过一锅法制备了木聚糖/聚乙烯醇/硼砂双网络水凝胶,表现出各种优异的性能,包括高强度(约 81kPa)、高韧性(约 1652.42kJ/m)、良好的自恢复性(约 79%的恢复)和优异的自修复性能(自修复效率达到 30s 时的 85.8%)。本研究提出了一种基于木聚糖设计高强度、高韧性、大拉伸性和自修复性能水凝胶的策略。

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