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铁电/铁弹性转变过程中的雪崩临界性。

Avalanche criticality during ferroelectric/ferroelastic switching.

作者信息

Casals Blai, Nataf Guillaume F, Salje Ekhard K H

机构信息

Department of Earth Sciences, Cambridge University, Cambridge, UK.

Department of Materials Science, Cambridge University, Cambridge, UK.

出版信息

Nat Commun. 2021 Jan 12;12(1):345. doi: 10.1038/s41467-020-20477-6.

Abstract

Field induced domain wall displacements define ferroelectric/ferroelastic hysteresis loops, which are at the core of piezoelectric, magnetoelectric and memristive devices. These collective displacements are scale invariant jumps with avalanche characteristics. Here, we analyse the spatial distribution of avalanches in ferroelectrics with different domain and transformation patterns: Pb(MgNb)O-PbTiO contains complex domains with needles and junction patterns, while BaTiO has parallel straight domains. Nevertheless, their avalanche characteristics are indistinguishable. The energies, areas and perimeters of the switched regions are power law distributed with exponents close to predicted mean field values. At the coercive field, the area exponent decreases, while the fractal dimension increases. This fine structure of the switching process has not been detected before and suggests that switching occurs via criticality at the coercive field with fundamentally different switching geometries at and near this critical point. We conjecture that the domain switching process in ferroelectrics is universal at the coercive field.

摘要

场致畴壁位移定义了铁电/铁弹滞回环,而这些滞回环是压电、磁电和忆阻器件的核心。这些集体位移是具有雪崩特性的尺度不变跳跃。在这里,我们分析了具有不同畴和相变模式的铁电体中雪崩的空间分布:Pb(MgNb)O-PbTiO包含具有针状和结状图案的复杂畴,而BaTiO具有平行的直畴。然而,它们的雪崩特性无法区分。开关区域的能量、面积和周长服从幂律分布,指数接近预测的平均场值。在 coercive 场,面积指数减小,而分形维数增加。这种开关过程的精细结构以前未被检测到,这表明开关是通过 coercive 场处的临界性发生的,在该临界点及附近具有根本不同的开关几何形状。我们推测铁电体中的畴开关过程在 coercive 场是普遍的。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7948/7804440/ab67d5c913d3/41467_2020_20477_Fig1_HTML.jpg

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