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压水堆模拟一回路水中质子辐照核级不锈钢的晶界氧化

Grain boundary oxidation of proton-irradiated nuclear grade stainless steel in simulated primary water of pressurized water reactor.

作者信息

Deng Ping, Peng Qunjia, Han En-Hou

机构信息

Nuclear Power Institute of China, Chengdu City, 610213, China.

Key Laboratory of Nuclear Materials and Safety Assessment, Institute of Metal Research, Chinese Academy of Sciences, Shenyang City, 110016, China.

出版信息

Sci Rep. 2021 Jan 14;11(1):1371. doi: 10.1038/s41598-020-80600-x.

DOI:10.1038/s41598-020-80600-x
PMID:33446760
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7809272/
Abstract

Grain boundary (GB) oxidation of proton-irradiated 304 nuclear grade stainless steel in primary water of pressurized water reactor was investigated. The investigation was conducted by studying microstructure of the oxide and oxide precursor formed at GB on an "atom-by-atom" basis by a combination of atom-probe tomography and transmission electron microscope. The results revealed that increasing irradiation dose promoted the GB oxidation, in correspondence with a different oxide and oxide precursor formed at the GB. Correlation of the oxide and oxide precursor with the GB oxidation behavior has been discussed in detail.

摘要

研究了质子辐照的304核级不锈钢在压水反应堆一回路水中的晶界(GB)氧化。通过结合原子探针断层扫描和透射电子显微镜,在“逐个原子”的基础上研究晶界处形成的氧化物和氧化物前驱体的微观结构来进行此项研究。结果表明,增加辐照剂量会促进晶界氧化,这与晶界处形成的不同氧化物和氧化物前驱体相对应。已详细讨论了氧化物和氧化物前驱体与晶界氧化行为的相关性。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/62b5fc99b09d/41598_2020_80600_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/542c2bf2cde1/41598_2020_80600_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/f933a53a20a3/41598_2020_80600_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/97d56b225bde/41598_2020_80600_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/dda26ca22ec0/41598_2020_80600_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/6d3c5cb64534/41598_2020_80600_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/62b5fc99b09d/41598_2020_80600_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/542c2bf2cde1/41598_2020_80600_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/f933a53a20a3/41598_2020_80600_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/97d56b225bde/41598_2020_80600_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/dda26ca22ec0/41598_2020_80600_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/6d3c5cb64534/41598_2020_80600_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b3ba/7809272/62b5fc99b09d/41598_2020_80600_Fig6_HTML.jpg

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